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Record W2115142031 · doi:10.1021/jp0129582

Enhancement of Red Emission (<sup>4</sup>F<sub>9/2</sub> → <sup>4</sup>I<sub>15/2</sub>) via Upconversion in Bulk and Nanocrystalline Cubic Y<sub>2</sub>O<sub>3</sub>:Er<sup>3+</sup>

2002· article· en· W2115142031 on OpenAlex

Why this work is in the frame

A frame that forgets how it found something cannot be audited. These are the routes that admitted this work.

affAt least one author lists a Canadian institution in the pinned OpenAlex snapshot.

Bibliographic record

VenueThe Journal of Physical Chemistry B · 2002
Typearticle
Languageen
FieldMaterials Science
TopicLuminescence Properties of Advanced Materials
Canadian institutionsConcordia University
Fundersnot available
KeywordsNanocrystalline materialPhoton upconversionDopantMaterials scienceAnalytical Chemistry (journal)ExcitationDopingIonEmission spectrumNanocrystalSpectral lineChemistryNanotechnologyOptoelectronicsPhysics

Abstract

fetched live from OpenAlex

In this paper, we investigate as a function of erbium concentration (1, 2, 5, 10 mol %) the upconversion properties of bulk and nanocrystalline Er 3+ doped cubic Y 2 O 3 . After excitation at short wavelength (488 nm) or with upconversion pumping (815 nm), green and red emissions were observed for both nanocrystalline and bulk samples in the visible region of the spectrum, while blue emission was observed in bulk Y 2 O 3:Er 3+ only. The upconverted emission after 815 nm excitation revealed an enhancement of the red [ 4 F 9/2 → 4 I 15/2 ] emission with respect to the green [( 2 H 11/2, 4 S 3/2 ) → 4 I 15/2 ] emission when the dopant concentration is increased. However, the magnitude of the red enhancement in the bulk material differs slightly from its nanocrystalline counterpart, with the nanocrystalline material showing a higher degree of dependence on the dopant Er 3+ concentration. It is believed that two distinct mechanisms are responsible for populating the 4 S 3/2 and 4 F 9/2 levels, with the latter being more efficient at higher Er 3+ ion concentration.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.002
metaresearch head score (Gemma)0.001
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesMeta-epidemiology (narrow)
Consensus categoriesMeta-epidemiology (narrow)
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.003
Threshold uncertainty score1.000

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0020.001
Meta-epidemiology (narrow)0.0020.001
Meta-epidemiology (broad)0.0030.001
Bibliometrics0.0000.001
Science and technology studies0.0010.001
Scholarly communication0.0000.002
Open science0.0020.001
Research integrity0.0010.001
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.010
GPT teacher head0.216
Teacher spread0.206 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it