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Record W2116338476

X-ray - Based Studies of Structural Dynamics in Solids and Liquids

2011· article· en· W2116338476 on OpenAlexfundno aff
R. Nüske

Bibliographic record

VenueLund University Publications (Lund University) · 2011
Typearticle
Languageen
FieldPhysics and Astronomy
TopicNuclear Physics and Applications
Canadian institutionsnot available
FundersVetenskapsrådetKnut och Alice Wallenbergs StiftelseDeutsche ForschungsgemeinschaftCarl Tryggers Stiftelse för Vetenskaplig ForskningNatural Sciences and Engineering Research Council of CanadaEuropean Commission
KeywordsPicosecondChemical physicsNanosecondWavelengthScatteringCrystal structureAtom (system on chip)PhysicsUltrashort pulseMoleculeStructure formationLaserMolecular physicsAtomic physicsOpticsCrystallographyChemistry
DOInot available

Abstract

fetched live from OpenAlex

The wavelength of x-ray radiation is much shorter than that of visible light. In fact, it is comparable to the distances between atoms in solids, which is on the order of one tenth of a nanometer. Using light of such a short wavelength, it is possible to study the structure of materials on the atom level. Scattering of x-rays has been developed into an invaluable tool to analyze various characteristics of matter, from the lattice structure of crystals to the structure of large biological molecules. In this way, we found that many of the properties of materials depend on their internal structure. To learn about changes in the structure of materials on the atom-level, time resolved x-ray scattering has proven a powerful technique. A wide variety of processes can be studied: from phase transitions in materials to vibrations in crystal lattices and pathways of chemical reactions. The aim of time-resolved studies is to follow these processes in real time. The timescale for changes in structure varies considerably depending on the underlying mechanism. Processes involving neighboring atoms typically take about 100\,fs. Structure changes involving large groups of atoms or molecules occure on a timescale of picoseconds to nanoseconds. Different mechanisms can be used to trigger changes in structure. Laser pulses with a duration of less than 100\,fs can be produced routinely and are used to initiate ultrafast changes in the structure. Alternatively, short electrical pulses can be used to trigger structural changes in piezo-electric materials. In this work, the main focus has been on experimental studies in order to deepen the understanding of structural changes in matter. The picosecond dynamics involved in the melting and recrystallization of a semiconductor, acoustic and thermal response of laser-excited solids, and the dynamics in the structure of a piezo-electric material have been studied. Additionally, instrumentation required for time-resolved x-ray scattering experiments has been developed.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.001
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.004
Threshold uncertainty score0.014

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.001
Meta-epidemiology (narrow)0.0010.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0010.001
Science and technology studies0.0010.001
Scholarly communication0.0010.002
Open science0.0010.001
Research integrity0.0010.001
Insufficient payload (model declined to judge)0.0040.001

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.023
GPT teacher head0.221
Teacher spread0.198 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations0
Published2011
Admission routes1
Has abstractyes

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