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Record W2117328675 · doi:10.1093/chromsci/44.4.219

Stacked Injection with Low Thermal Mass Gas Chromatography for PPB Level Detection of Oxygenated Compounds in Hydrocarbons

2006· article· en· W2117328675 on OpenAlex

Why this work is in the frame

A frame that forgets how it found something cannot be audited. These are the routes that admitted this work.

affAt least one author lists a Canadian institution in the pinned OpenAlex snapshot.

Bibliographic record

VenueJournal of Chromatographic Science · 2006
Typearticle
Languageen
FieldChemistry
TopicAnalytical Chemistry and Chromatography
Canadian institutionsDow Chemical (Canada)
FundersDow Chemical Company
KeywordsChemistryChromatographyGas chromatographyHydrocarbonOrganic chemistry

Abstract

fetched live from OpenAlex

The presence of oxygenated compounds in light hydrocarbons can have a negative impact in manufacturing processes and on the quality of products produced. The development of an analytical technique termed "stacked injection" has been reported earlier. With this technique, sensitivity in the parts-per-billion (ppb) range for oxygenated compounds can be achieved, even with a flame ionization detector; however, there are drawbacks for this approach that limit its overall effectiveness. A new, improved analytical technique has been developed that not only addresses the shortcomings encountered, but offers markedly higher analytical performance. The new concept employs multidimensional gas chromatography (GC) with low thermal mass GC. With this new approach, throughput improvements of up to 5 times, range extension of solutes amenable for this analysis of up to nC16 alcohol, and ppb levels of detection for oxygenated compounds are achieved. Apart from alcohols, this technique is successfully employed for the ppb level analysis of other classes of oxygenated compounds, such as ethers, aldehydes, and aromatics.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.001
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesMeta-epidemiology (narrow)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.011
Threshold uncertainty score1.000

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0010.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0010.000
Bibliometrics0.0010.004
Science and technology studies0.0000.001
Scholarly communication0.0000.001
Open science0.0010.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.009
GPT teacher head0.222
Teacher spread0.213 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it