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High‐Temperature Neutron Diffraction of the AlN–Al <sub>2</sub> O <sub>3</sub> –Y <sub>2</sub> O <sub>3</sub> System

2003· article· en· W2123271635 on OpenAlexaff
Mamoun Medraj, Robert P. Hammond, R. A. L. Drew

Bibliographic record

VenueJournal of the American Ceramic Society · 2003
Typearticle
Languageen
FieldMaterials Science
TopicAdvanced ceramic materials synthesis
Canadian institutionsMcGill UniversityRoyal Military College of CanadaNational Research Council CanadaConcordia University
Fundersnot available
KeywordsMaterials sciencePhase diagramTernary operationNitrideAtmospheric temperature rangeTernary numeral systemPhase (matter)Analytical Chemistry (journal)ThermodynamicsNeutron diffractionCrystallographyComposite materialCrystal structureChemistry

Abstract

fetched live from OpenAlex

The importance of aluminum nitride (AlN) stems from its application in microelectronics as a substrate material due to high thermal conductivity, high electrical resistance, mechanical strength and hardness, thermal durability, and chemical stability. Yttria (Y 2 O 3 ) is the best additive for AlN sintering. AlN densifies by a liquid‐phase mechanism, where the surface oxide, Al 2 O 3 , reacts with Y 2 O 3 to form an Y‐Al‐O‐N liquid that promotes particle rearrangement and densification. Construction of the phase relations in this multicomponent system is essential for optimizing the properties of AlN. The ternary phase diagram of the AlN–Al 2 O 3 –Y 2 O 3 was developed by Gibbs energy minimization using interpolation procedures based on modeling the binary subsystems. This paper aims at testing the resultant understanding experimentally at selected compositions using in situ high‐temperature neutron diffractometry. These experimental results agree with the thermodynamic calculations of AlN–Al 2 O 3 –Y 2 O 3 . The ternary phase diagram has been constructed for the first time in this work. High‐temperature neutron diffractometry has permitted real time measurement of the reactions involved in this ternary system, especially to determine the temperature range for each reaction, which would have been difficult to establish by other means.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.003
Threshold uncertainty score0.007

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.006
GPT teacher head0.213
Teacher spread0.207 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations14
Published2003
Admission routes1
Has abstractyes

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Same venueJournal of the American Ceramic SocietySame topicAdvanced ceramic materials synthesisFrench-language works237,207