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Record W2123841027 · doi:10.1139/t99-106

The role of clay minerals and the effect of H<sup>+</sup> ions on removal of heavy metal (Pb<sup>2+</sup>) from contaminated soils

2000· article· en· W2123841027 on OpenAlex

Why this work is in the frame

A frame that forgets how it found something cannot be audited. These are the routes that admitted this work.

fundA Canadian funder is recorded on the work.
venuePublished in a venue whose home country is Canada.
no affNo Canadian affiliation: this work is invisible to an affiliation-only frame.
No Canadian affiliation. An affiliation-only frame, the usual design, would never have seen this work. It is one of the works that make the case for inverting the frame.

Bibliographic record

VenueCanadian Geotechnical Journal · 2000
Typearticle
Languageen
FieldEngineering
TopicElectrokinetic Soil Remediation Techniques
Canadian institutionsnot available
FundersUniversity of British Columbia
KeywordsKaoliniteIlliteClay mineralsChemistryAdsorptionSorptionDesorptionMetal ions in aqueous solutionSurface chargeInorganic chemistrySoil waterDissolutionMetalMineralogyGeologySoil science

Abstract

fetched live from OpenAlex

The importance of the surface charge of clay minerals (fixed or variable) and the effect of H + ions on the adsorption and removal of Pb 2+ ions from contaminated soil are investigated using kaolinite (variable charge) and two illitic (fixed charge) soils with pH 3.9 and 9.2. The adsorption-desorption characteristics of Pb 2+ ions were determined using batch equilibrium tests and acid leach tests with various acids used to leach the soils. Under the same adsorption conditions, illitic soil adsorbed much more Pb 2+ ions than kaolinite. The difference is largely due to the surface charges on the clay minerals. Removal of Pb 2+ ions from variable-charge minerals (e.g., kaolinite) requires much less effort than removal of Pb 2+ ions from constant-charge minerals (e.g., illite). The surface charge of a clay mineral has an important effect. By increasing the number of H + ions available in the soil system with a buffer solution such as NaOAc-HOAc, heavy metals adsorbed on the clay surface are expelled to pore water. The increase in H + ions in the soil system also assists in dissolving any metal carbonates, thereby increasing the solubility of heavy metals in illitic soil. The more H + ions available in the pore fluid, the more Pb 2+ ions can be released from the system.Key words: clay minerals, sorption, desorption, heavy metal, hydrogen ion, electrokinetic, acid leach.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.001
metaresearch head score (Gemma)0.001
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Simulation or modeling · Consensus signal: none
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.512
Threshold uncertainty score0.999

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0010.001
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0010.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.001
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.003
GPT teacher head0.194
Teacher spread0.191 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it