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The Cross‐Dehydrogenative Coupling of CH Bonds: A Versatile Strategy for CC Bond Formations

2013· article· en· 1,848 citations· W2128434938 on OpenAlex· 10.1002/anie.201304268

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Opus teacher head0.030
GPT teacher head0.318
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Validation status
score_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Abstract

Over the last decade, substantial research has led to the introduction of an impressive number of efficient procedures which allow the selective construction of CC bonds by directly connecting two different CH bonds under oxidative conditions. Common to these methodologies is the generation of the reactive intermediates in situ by activation of both CH bonds. This strategy was introduced by the group of Li as cross-dehydrogenative coupling (CDC) and discloses waste-minimized synthetic alternatives to classic coupling procedures which rely on the use of prefunctionalized starting materials. This Review highlights the recent progress in the field of cross-dehydrogenative C sp 3C formations and provides a comprehensive overview on existing procedures and employed methodologies.

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The record

Venue
Angewandte Chemie International Edition
Topic
Catalytic C–H Functionalization Methods
Field
Chemistry
Canadian institutions
McGill UniversityCentre in Green Chemistry and Catalysis
Funders
Keywords
BondCoupling (piping)Combinatorial chemistryChemistryNanotechnologyComputer scienceMaterials scienceEngineeringBusinessMechanical engineering
Has abstract in OpenAlex
yes