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Record W2128844784 · doi:10.1680/gmat.12.00012

Redispersing aggregated latexes made with switchable surfactants

2012· article· en· W2128844784 on OpenAlex

Why this work is in the frame

A frame that forgets how it found something cannot be audited. These are the routes that admitted this work.

affAt least one author lists a Canadian institution in the pinned OpenAlex snapshot.
fundA Canadian funder is recorded on the work.

Bibliographic record

VenueGreen Materials · 2012
Typearticle
Languageen
FieldChemistry
TopicAdvanced Polymer Synthesis and Characterization
Canadian institutionsQueen's University
FundersCanada Research Chairs
KeywordsEmulsion polymerizationDewateringMaterials sciencePolystyreneMethyl methacrylateEmulsionPotassium persulfateChemical engineeringPolymerSonicationDepolymerizationPolymerizationWaste managementPolymer chemistryComposite material

Abstract

fetched live from OpenAlex

Amidine-based switchable surfactants can be used as stabilizers during emulsion polymerization, and the resulting latexes can then be destabilized simply by the removal of CO 2 . Polystyrene and poly(methyl methacrylate [MMA]) latexes have been successfully redispersed by reintroducing CO 2 to the latex, as shown by recovery of primary particle size, but an input of energy was required. Sonication is the most effective method of energy input, but lower-energy methods, such as rotor–stators and a blender, are successful in redispersing some aggregated latexes. Colloidal stability was found to be reversible for at least three aggregation/redispersion cycles, and redispersibility was achieved even after the removal of water and addition of fresh water. The traditional method of aggregating latexes involves addition of salts, acids or bases, which result in a contaminated wastewater stream. Furthermore, aggregated latexes cannot usually be redispersed. This approach could enable dewatering of latexes prior to transport followed by redispersion at the point of use, yielding significantly reduced transportation costs and energy consumption.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesInsufficient payload (model declined to judge)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.005
Threshold uncertainty score0.996

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0050.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.013
GPT teacher head0.217
Teacher spread0.204 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it