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Instabilities in thin polymer films: from pattern formation to rupture

2000· article· en· W2138365163 on OpenAlex

Why this work is in the frame

A frame that forgets how it found something cannot be audited. These are the routes that admitted this work.

affAt least one author lists a Canadian institution in the pinned OpenAlex snapshot.

Bibliographic record

VenueMacromolecular Symposia · 2000
Typearticle
Languageen
FieldPhysics and Astronomy
TopicForce Microscopy Techniques and Applications
Canadian institutionsUniversity of Guelph
Fundersnot available
Keywordsvan der Waals forceThin filmPolystyrenePolymerMaterials scienceAnnealing (glass)Composite materialChemical physicsNanotechnologyMoleculeChemistryOrganic chemistry

Abstract

fetched live from OpenAlex

Thermal fluctuations of the surfaces of thin polymer films can be amplified by the long-range van der Waals or dispersion force which acts across the film. When freely-standing polymer films are heated, this instability leads to the formation of holes. We have measured the formation and growth of holes in very thin, freely-standing polystyrene (PS) films to learn about the mobility of the confined polymer molecules. We have also symmetrically capped freely-standing PS films with thin, solid layers to probe the effects of mechanical confinement. Aggressive annealing of the trilayer films produces a novel in-plane morphology which can be understood in terms of the balance between the decrease in free energy associated with the dispersion interaction and the increase in free energy associated with the bending of the capping layers. The general nature of the morphology, and its reversibility, is demonstrated.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesInsufficient payload (model declined to judge)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.097
Threshold uncertainty score0.998

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0030.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.003
GPT teacher head0.226
Teacher spread0.223 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it