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Record W2143294131 · doi:10.1002/qua.21983

Coordinate scaling of the kinetic energy in pair density functional theory: A Legendre transform approach

2009· article· en· W2143294131 on OpenAlexaff
Rogelio Cuevas‐Saavedra, Paul W. Ayers

Bibliographic record

VenueInternational Journal of Quantum Chemistry · 2009
Typearticle
Languageen
FieldPhysics and Astronomy
TopicSpectroscopy and Quantum Chemical Studies
Canadian institutionsMcMaster University
Fundersnot available
KeywordsLegendre transformationLegendre polynomialsScalingDensity functional theoryLegendre functionAssociated Legendre polynomialsKinetic energyHomogeneousOrbital-free density functional theoryStatistical physicsQuantumMathematicsApplied mathematicsPhysicsMathematical analysisHybrid functionalQuantum mechanicsGeometryOrthogonal polynomials

Abstract

fetched live from OpenAlex

Abstract We show that the kinetic energy functional in pair density functional theory is homogeneous of degree 2 with respect to coordinate scaling. Although this result was already derived by Levy and Ziesche using the constrained search method (Levy and Ziesche, J Chem Phys 2001, 115, 9110 ), we derive our result using the Legendre transform formulation (Ayers et al., J Chem Phys 2006, 124, 054101 ). The advantage of this approach is that in the Legendre transform functional, the N ‐representability problem is solved by the functional. By contrast, in the Levy–Ziesche approach, the computationally impracticable N ‐representability constraints have to be imposed separately. © 2009 Wiley Periodicals, Inc. Int J Quantum Chem, 2009

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.159
Threshold uncertainty score0.362

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.009
GPT teacher head0.232
Teacher spread0.223 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations17
Published2009
Admission routes1
Has abstractyes

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