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Record W2147092973 · doi:10.1080/00218460490480824

A NEW MODEL FOR THE ELECTRICAL DOUBLE LAYER INTERACTION BETWEEN TWO SURFACES IN AQUEOUS SOLUTIONS

2004· article· en· W2147092973 on OpenAlexaff
Carolyn L. Ren, Yandong Hu, Dongqing Li, Carsten Werner

Bibliographic record

VenueThe Journal of Adhesion · 2004
Typearticle
Languageen
FieldEngineering
TopicMicrofluidic and Bio-sensing Technologies
Canadian institutionsUniversity of Toronto
Fundersnot available
KeywordsOsmotic coefficientAqueous solutionIonic bondingPoisson–Boltzmann equationCounterionThermodynamicsInteraction energyMaterials scienceIonOsmotic pressureActivity coefficientNernst equationChemistryStatistical physicsPhysicsPhysical chemistryMolecule

Abstract

fetched live from OpenAlex

A new theoretical model is developed to evaluate the total potential energy of interaction between two charged flat plates in aqueous solutions. Instead of using the Boltzmann distribution to predict the ionic concentrations of counterion and coion, which is not correct for small confined spaces, this modified model determines the ionic concentrations of counterion and coion based on the Poisson equation, the Nernst equation, and the mass conservation condition. Instead of the approximations used in the traditional model, the osmotic pressure is directly evaluated based on the ionic concentration distributions predicted by this new model. Finally, the total interaction energy is examined and compared with that predicted by the traditional model. It has been found that for high ionic concentration solutions, the traditional model tends to overestimate the total interaction energy due to the approximations employed in simplifying the osmotic pressure. However, for dilute solutions, the traditional model tends to underestimate the total interaction energy at small separation distance due to the misuse of the Boltzmann distribution in calculating the ionic concentration.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.001
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Theoretical or conceptual · Consensus signal: none
GenreCandidate signal: Methods · Consensus signal: Methods
Teacher disagreement score0.004
Threshold uncertainty score0.013

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.001
Meta-epidemiology (narrow)0.0010.001
Meta-epidemiology (broad)0.0010.001
Bibliometrics0.0010.001
Science and technology studies0.0010.001
Scholarly communication0.0010.003
Open science0.0030.001
Research integrity0.0030.001
Insufficient payload (model declined to judge)0.0040.001

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.060
GPT teacher head0.285
Teacher spread0.225 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designTheoretical or conceptual
Domainnot available
GenreMethods

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations14
Published2004
Admission routes1
Has abstractyes

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