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Record W2154339480 · doi:10.1139/v04-034

High-resolution terahertz spectrum of CH<sub>2</sub> Low <i>J</i> rotational transitions near 2 THz

2004· article· en· W2154339480 on OpenAlexvenueno aff
Sandra Brünken, E A Michael, Frank Lewen, T. F. Giesen, Hiroyuki Ozeki, G. Winnewisser, Per Jensen, Eric Herbst

Bibliographic record

VenueCanadian Journal of Chemistry · 2004
Typearticle
Languageen
FieldChemistry
TopicMolecular Spectroscopy and Structure
Canadian institutionsnot available
FundersOhio State UniversityDeutsche ForschungsgemeinschaftNational Aeronautics and Space Administration
KeywordsHyperfine structureTerahertz radiationChemistryMultipletMethyleneGround stateRotational spectrumSpectroscopyRotational transitionAtomic electron transitionSpectral lineAtomic physicsRotational spectroscopyMolecular electronic transitionMolecular physicsMoleculePhysicsOptics

Abstract

fetched live from OpenAlex

The methylene radical (CH 2 ) was very important to Gerhard Herzberg. We have carried out high-resolution spectroscopic measurements on two energetically low-lying, pure rotational transitions of methylene in its ground vibrational–electronic state at frequencies near 2 THz. One of the transitions — the N KaKc = 2 11 ← 2 02 multiplet — belongs to ortho-CH 2 and is centered at 1.954 THz. The other rotational transition — the N KaKc = 1 10 ← 1 01 multiplet — belongs to para-CH 2 and is centered at 1.915 THz. Since the ground electronic state of methylene has 3 B 1 symmetry, the rotational transitions are split into three fine-structure components, while the ortho transitions are split additionally by hyperfine structure. In total, we have measured 29 new lines, six for the para transition and the remainder for the ortho transition. The newly measured lines can be added to high-resolution spectral data obtained by ourselves and others at lower frequencies. Progress towards a global fit is discussed. Key words: spectroscopy, THz frequencies, radicals, methylene, interstellar medium.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesInsufficient payload (model declined to judge)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.004
Threshold uncertainty score1.000

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.001
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.003
GPT teacher head0.177
Teacher spread0.174 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations17
Published2004
Admission routes1
Has abstractyes

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