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Record W2154959666 · doi:10.1002/cjce.5450810353

Oxidation of Tetrachloroethylene in a Bubble Column Photochemical Reactor Applying the UV/H<sub>2</sub>O<sub>2</sub> Technique

2003· article· en· W2154959666 on OpenAlexvenueno aff
Dzevo Alibegic, Satoshi Tsuneda, Akira Hirata

Bibliographic record

VenueThe Canadian Journal of Chemical Engineering · 2003
Typearticle
Languageen
FieldEnvironmental Science
TopicAdvanced oxidation water treatment
Canadian institutionsnot available
Fundersnot available
KeywordsTetrachloroethyleneChemistryMass transferReaction rate constantBubble column reactorAnalytical Chemistry (journal)KineticsMass transfer coefficientBubbleAbsorption (acoustics)PhotochemistryChromatographyMaterials scienceOrganic chemistryGas bubble

Abstract

fetched live from OpenAlex

Abstract Mass transfer of tetrachloroethylene (PCE) gas, followed by a free‐OH radical reaction in the liquid phase, was studied in a bubble column reactor equipped with a UV light source and containing aqueous H 2 O 2 as the reacting medium. Degradation of PCE in the liquid phase was found to follow pseudo‐first‐order kinetics, and the optimal ratio of H 2 O 2 /PCE leading to the highest oxidation rate could be successfully obtained from the analysis of the steady‐state OH radical concentration. Absorption of PCE gas was in the kinetic slow regime and could be predicted based on the ratio of the apparent rate constant of PCE liquid degradation to the volumetric mass transfer coefficient ( kapp/K L a ). The presence of small amounts of PCE in the liquid bulk had positive effect on the mass transfer over the range studied and need to be taken into account.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.001
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.005
Threshold uncertainty score0.592

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0010.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.001
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.006
GPT teacher head0.185
Teacher spread0.179 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations4
Published2003
Admission routes1
Has abstractyes

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