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Record W2155436602 · doi:10.1089/109287503763336566

Droplet Combustion of Chlorinated Benzenes, Alkanes, and Their Mixtures in a Dry Atmosphere

2003· article· en· W2155436602 on OpenAlexaff
W.J. Stry, James D. Felske, Nasser Ashgriz

Bibliographic record

VenueEnvironmental Engineering Science · 2003
Typearticle
Languageen
FieldEngineering
TopicParticle Dynamics in Fluid Flows
Canadian institutionsUniversity of Toronto
Fundersnot available
KeywordsChlorobenzeneAtmosphere (unit)ChemistryDecaneCombustionHexadecaneAlkaneVaporizationHydrogenVolatilisationAnalytical Chemistry (journal)Yield (engineering)Environmental chemistryThermodynamicsHydrocarbonOrganic chemistry

Abstract

fetched live from OpenAlex

Combustion of three chlorobenzenes (monochlorobenzene, dichlorobenzene, trichlorobenzene) and five alkanes (octane, decane, dodecane, tetradecane, and hexadecane) were investigated. Using high-speed video photography, the size and velocity of the burning drops at various points during their lifetime were measured. From such data, the time-variation of a droplet's burning rate was deduced. It was found that the variations of the burning rates for the mixtures were qualitatively similar when viewed as functions of the chlorine to hydrogen atom ratio. Starting from a pure alkane, as Cl/H increased, the burning rate first decreased, then slightly increased, and then fell sharply near Cl/H = 0.5 to approximately the vaporization rate of the pure chlorobenzene. It was also found that prior droplet combustion studies (performed in the H2O-rich atmosphere of combustion-heated reactors) exhibited burning rates of the same liquid blends that were nearly twice the present dry atmosphere results. We have demonstrated that when the hydrogen in the surrounding atmospheric H2O is included in the ratio Cl/H, these previous results yield curves of burning rate vs. Cl/H that are similar to those of the present study. This implies that the enhanced burning rate observed when an alkane is blended into a pure chlorobenzene is partly due to the hydrogen provided by the alkane, and that a similar effect appears achievable by adding water vapor to the gas phase.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.001
Threshold uncertainty score0.003

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.003
GPT teacher head0.163
Teacher spread0.160 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations4
Published2003
Admission routes1
Has abstractyes

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