MétaCan
Menu
Back to cohort
Record W2160876051 · doi:10.5194/acp-14-3373-2014

On the temperature dependence of organic reactivity, nitrogen oxides, ozone production, and the impact of emission controls in San Joaquin Valley, California

2014· article· en· W2160876051 on OpenAlexaff
Sally E. Pusede, Drew R. Gentner, P. J. Wooldridge, E. C. Browne, Andrew W. Rollins, K.‐E. Min, A. R. Russell, Jordan Thomas, L. Zhang, W. H. Brune, S. B. Henry, Joshua P. DiGangi, Frank N. Keutsch, S. A. Harrold, Joel A. Thornton, M. R. Beaver, Jason M. St. Clair, P. O. Wennberg, John E. Sanders, Xinrong Ren, Trevor C. VandenBoer, M. Z. Markovic, A. Guha, R. J. Weber, Allen H. Goldstein, R. C. Cohen

Bibliographic record

VenueAtmospheric chemistry and physics · 2014
Typearticle
Languageen
FieldEarth and Planetary Sciences
TopicAtmospheric chemistry and aerosols
Canadian institutionsUniversity of Toronto
FundersCalifornia Air Resources BoardNational Aeronautics and Space Administration
KeywordsSan JoaquinNOxOzoneEnvironmental scienceAir quality indexAtmospheric sciencesVolatile organic compoundNitrogen oxidesNitrogen oxideEnvironmental chemistryDaytimeChemistryMeteorologyGeographyWaste management

Abstract

fetched live from OpenAlex

Abstract. The San Joaquin Valley (SJV) experiences some of the worst ozone air quality in the US, frequently exceeding the California 8 h standard of 70.4 ppb. To improve our understanding of trends in the number of ozone violations in the SJV, we analyze observed relationships between organic reactivity, nitrogen oxides (NOx), and daily maximum temperature in the southern SJV using measurements made as part of California at the Nexus of Air Quality and Climate Change in 2010 (CalNex-SJV). We find the daytime speciated organic reactivity with respect to OH during CalNex-SJV has a temperature-independent portion with molecules typically associated with motor vehicles being the major component. At high temperatures, characteristic of days with high ozone, the largest portion of the total organic reactivity increases exponentially with temperature and is dominated by small, oxygenated organics and molecules that are unidentified. We use this simple temperature classification to consider changes in organic emissions over the last and next decade. With the CalNex-SJV observations as constraints, we examine the sensitivity of ozone production (PO3) to future NOx and organic reactivity controls. We find that PO3 is NOx-limited at all temperatures on weekends and on weekdays when daily maximum temperatures are greater than 29 °C. As a consequence, NOx reductions are the most effective control option for reducing the frequency of future ozone violations in the southern SJV.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.211
Threshold uncertainty score0.603

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.005
GPT teacher head0.196
Teacher spread0.191 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations133
Published2014
Admission routes1
Has abstractyes

Explore more

Same venueAtmospheric chemistry and physicsSame topicAtmospheric chemistry and aerosolsFrench-language works237,207