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Record W2164427272

Practical Aspects of Modern Routine Solid-State Multinuclear Magnetic Resonance Spectroscopy: One-Dimensional Experiments

2001· article· en· W2164427272 on OpenAlexaff
David L. Bryce, Guy M. Bernard, Myrlene Gee, Michael D. Lumsden, Klaus Eichele, Roderick E. Wasylishen

Bibliographic record

Venuenot available
Typearticle
Languageen
FieldChemistry
TopicAdvanced NMR Techniques and Applications
Canadian institutionsUniversity of Alberta
Fundersnot available
KeywordsSolid-state nuclear magnetic resonanceSolid-stateVariety (cybernetics)DeuteriumMaterials scienceNanotechnologyChemistryNuclear magnetic resonanceComputer sciencePhysicsPhysical chemistryNuclear physicsArtificial intelligence
DOInot available

Abstract

fetched live from OpenAlex

New solid-state NMR (SSNMR) methods and applications continue to blossom such that a diverse array of physical, chemical, and biological problems are now being addressed using a variety of SSNMR experiments. While SSNMR is far from routine for chemists in the manner that a technique such as solution NMR is, there are nevertheless numerous applications of SSNMR which would be beneficial to many “non-specialists”, e.g., synthetic chemists seeking to characterize their materials. This article gathers together practical details for those one-dimensional experiments which, in a broad sense, are considered “routine ” in a modern SSNMR laboratory. Emphasis is placed on providing information and over 300 key references in a manner which will be useful for the novice and the non-specialist. For practicing SSNMR spectroscopists, it is hoped that this article will serve as a valuable reference in the laboratory. In addition to providing a brief review of pulsed Fourier transform NMR, the article discusses experimental details relating to the study of solid samples containing spin- 1 2 nuclei, non-integer quadrupolar nuclei, and deuterium.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.008
metaresearch head score (Gemma)0.010
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Not applicable · Consensus signal: none
GenreCandidate signal: Methods · Consensus signal: Methods
Teacher disagreement score0.008
Threshold uncertainty score0.043

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0080.010
Meta-epidemiology (narrow)0.0010.001
Meta-epidemiology (broad)0.0010.000
Bibliometrics0.0010.001
Science and technology studies0.0010.004
Scholarly communication0.0020.005
Open science0.0030.003
Research integrity0.0030.004
Insufficient payload (model declined to judge)0.0050.003

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.029
GPT teacher head0.345
Teacher spread0.315 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designNot applicable
Domainnot available
GenreMethods

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations78
Published2001
Admission routes1
Has abstractyes

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Same topicAdvanced NMR Techniques and ApplicationsFrench-language works237,207