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Record W2166825986 · doi:10.1029/2004wr003157

Origin and migration of dissolved organic carbon fractions in a clay‐rich aquitard: <sup>14</sup>C and δ<sup>13</sup>C evidence

2005· article· en· W2166825986 on OpenAlexafffund
M. Jim Hendry, Leonard I. Wassenaar

Bibliographic record

VenueWater Resources Research · 2005
Typearticle
Languageen
FieldEarth and Planetary Sciences
TopicGroundwater and Isotope Geochemistry
Canadian institutionsGlobal Institute for Water SecurityEnvironment and Climate Change CanadaUniversity of Saskatchewan
FundersNatural Sciences and Engineering Research Council of CanadaCameco
KeywordsDissolved organic carbonAquiferPore water pressureTotal organic carbonChemistryDiffusionCarbon fibersSoil scienceGeologyEnvironmental chemistryAnalytical Chemistry (journal)MineralogyGroundwaterMaterials scienceThermodynamics

Abstract

fetched live from OpenAlex

The origin and long‐term transport of dissolved organic carbon (DOC) and its high molecular weight (HMW) and low molecular weight (LMW) fractions were investigated in a clay‐rich till aquitard system. DOC concentrations decreased systematically with depth from 168 mg L −1 in the surficial fractured zone (1.2 m) to minimum values of 12–16 mg L −1 from 15 to 43 m depth in the nonfractured aquitard. The HMW and LMW DOC fractions and their corresponding δ 13 C values also decreased systematically with depth. Numerical transport simulations of the downward migration of DOC from the soil zone into the aquitard closely approximated field‐measured values and show transport of DOC was controlled by diffusive mixing. The depth trends for HMW and LMW DOC fractions and δ 13 C support hypothesized transport via diffusion, as well as earlier findings that microbial respiration in this nonfractured aquitard was negligible over the time period studied. The 14 C content of the HMW DOC fraction decreased systematically with depth from 87 percent modern carbon (pmC) at 1.2 m to 13–15 pmC from 15 to 43 m depth. A simple model accounting for diffusive mixing and radioactive decay described the 14 C profile in the aquitard. Radiocarbon measurements, transport modeling, and δ 13 C data suggest DOC and its fractions were derived from two distinct end‐members: soil organic carbon formed since the Holocene (∼10 ka B.P.) and DOC in connate pore water (∼15 ka B.P.).

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.001
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Observational · Consensus signal: Observational
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.392
Threshold uncertainty score0.992

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0010.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.001
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.037
GPT teacher head0.285
Teacher spread0.248 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designObservational
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations38
Published2005
Admission routes2
Has abstractyes

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