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Electron paramagnetic resonance of individual atoms on a surface

2015· article· en· 421 citations· W2175801878 on OpenAlex· 10.1126/science.aac8703

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Canadian funderA Canadian agency funded it. The work may carry no Canadian affiliation at all.

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Opus teacher head0.017
GPT teacher head0.255
Teacher spread
0.238 · how far apart the two teachers sit on this one work
Validation status
score_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Abstract

We combined the high-energy resolution of conventional spin resonance (here ~10 nano-electron volts) with scanning tunneling microscopy to measure electron paramagnetic resonance of individual iron (Fe) atoms placed on a magnesium oxide film. We drove the spin resonance with an oscillating electric field (20 to 30 gigahertz) between tip and sample. The readout of the Fe atom's quantum state was performed by spin-polarized detection of the atomic-scale tunneling magnetoresistance. We determine an energy relaxation time of T1 ≈ 100 microseconds and a phase-coherence time of T2 ≈ 210 nanoseconds. The spin resonance signals of different Fe atoms differ by much more than their resonance linewidth; in a traditional ensemble measurement, this difference would appear as inhomogeneous broadening.

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The record

Venue
Science
Topic
Quantum and electron transport phenomena
Field
Physics and Astronomy
Canadian institutions
Funders
Office of Naval ResearchEngineering and Physical Sciences Research CouncilNatural Sciences and Engineering Research Council of Canada
Keywords
NanosecondResonance (particle physics)Laser linewidthElectron paramagnetic resonanceMicrosecondAtom (system on chip)Atomic physicsChemistryQuantum tunnellingCondensed matter physicsElectronRelaxation (psychology)Spin (aerodynamics)Materials scienceNuclear magnetic resonancePhysicsLaserOptics
Has abstract in OpenAlex
yes