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Record W2175865729 · doi:10.1021/bk-2013-1124.ch013

Dye-Sensitized Photocatalyst: A Breakthrough in Green Energy and Environmental Detoxification

2013· book-chapter· en· W2175865729 on OpenAlexaff
Pankaj Chowdhury, Hassan Gomaa, Ajay K. Ray

Bibliographic record

VenueACS symposium series · 2013
Typebook-chapter
Languageen
FieldEnergy
TopicAdvanced Photocatalysis Techniques
Canadian institutionsWestern University
Fundersnot available
KeywordsPhotocatalysisPhotochemistryMaterials scienceVisible spectrumElectron transferPhotodegradationChemistryOrganic chemistryCatalysisOptoelectronics

Abstract

fetched live from OpenAlex

Sensitization of semiconductor material is well recognized in the field of photography and photo-electrochemistry. Recently, dye sensitization technique has found its application in solar cells. Dye sensitization can further be applied for water treatment and sacrificial hydrogen generation using photocatalysis. Success of the process depends on the choice of suitable dye, semiconductor material, electron donor, and light sources. Attachment of dye molecule on photocatalyst surface leads to subsequent electron transfer into the conduction band of semiconductor, therefore strongly bound anchoring groups are preferred. Fixation of dye molecule on semiconductor surface also improves the electron transfer process. Incorporation of noble metals on semiconductor surface enhances their photocatalytic activity by reducing the electron/hole recombination rate. Dye-sensitized photocatalyst is applied for degradation of a wide range of compounds such as i) aliphatic compounds (carbon tetrachloride, trichloroethylene, hydrazine, and pesticides), ii) aromatic compounds (non-sensitizing dye, phenol, chlorophenol, and benzyl alcohol) in aqueous medium. Hydrogen generation is also possible in visible light with dye-sensitized photocatalyst in presence of sacrificial reagents. Ruthenium based dyes in solar cells and dye-sensitized photocatalysis are the best reported so far, however, researchers are gradually switching towards inexpensive and environment-friendly organic dyes and/or natural dyes from vegetable sources. Eosin Y is an organic dye which has been widely used for hydrogen generation, reportedly providing quantum yields between 9-19 %.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Theoretical or conceptual · Consensus signal: none
GenreCandidate signal: Other · Consensus signal: none
Teacher disagreement score0.002
Threshold uncertainty score0.007

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0010.000
Meta-epidemiology (broad)0.0010.000
Bibliometrics0.0010.001
Science and technology studies0.0000.000
Scholarly communication0.0010.001
Open science0.0010.001
Research integrity0.0010.002
Insufficient payload (model declined to judge)0.0020.002

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.008
GPT teacher head0.203
Teacher spread0.196 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designTheoretical or conceptual
Domainnot available
GenreOther

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations37
Published2013
Admission routes1
Has abstractyes

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