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Record W2186824350 · doi:10.2138/am-2015-5336

Direct and indirect evidence for free oxygen (O <sup>2−</sup> ) in MO-silicate glasses and melts (M = Mg, Ca, Pb)

2015· article· en· W2186824350 on OpenAlex

Why this work is in the frame

A frame that forgets how it found something cannot be audited. These are the routes that admitted this work.

affAt least one author lists a Canadian institution in the pinned OpenAlex snapshot.

Bibliographic record

VenueAmerican Mineralogist · 2015
Typearticle
Languageen
FieldMaterials Science
TopicGlass properties and applications
Canadian institutionsUniversity of TorontoWestern University
FundersNational Science Council
KeywordsSilicateOxygenNatural bond orbitalX-ray photoelectron spectroscopyAnalytical Chemistry (journal)OxideChemistryIonOxygen atomInorganic chemistryMineralogyDensity functional theoryNuclear magnetic resonanceMoleculePhysicsComputational chemistryEnvironmental chemistry

Abstract

fetched live from OpenAlex

Oxygen 1s XPS spectra of a Pb-silicate glass containing 76.6 mol% PbO provide the first accurate, direct measurement of free oxide ion (O2-) in these glasses. O2- constitutes 35 (±3) mol% of total oxygen, with NBO and BO constituting, respectively, 52 (±3) and 13 (±3) mol%. All 29Si NMR and O 1s XPS results for Pb-silicate glasses indicate mol% levels of O2- containing more than ~30 mol% PbO. The O2- abundances are consistent with equilibrium thermodynamic considerations where K ~ 12 for the mass action equation involving NBO, BO, and O2-.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.001
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: none
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.622
Threshold uncertainty score0.993

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.001
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.001
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.073
GPT teacher head0.305
Teacher spread0.232 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it