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Behavior and characterization of titanium dioxide and silver nanoparticles in soils

2015· review· en· W2210135262 on OpenAlexafffund
Vinayak Laxman Pachapur, Araceli Dalila Larios, Maximiliano Cledón, Satinder Kaur Brar, Mausam Verma, Rao Y. Surampalli

Bibliographic record

VenueThe Science of The Total Environment · 2015
Typereview
Languageen
FieldMaterials Science
TopicNanoparticles: synthesis and applications
Canadian institutionsInstitut National de la Recherche Scientifique
FundersNatural Sciences and Engineering Research Council of CanadaMinistère de l'Agriculture, des Pêcheries et de l'Alimentation
KeywordsDissolutionSoil waterZeta potentialTitanium dioxideBioavailabilityEnvironmental chemistryClay mineralsCharacterization (materials science)ChemistryEconomies of agglomerationMatrix (chemical analysis)Chemical engineeringMaterials scienceEnvironmental scienceNanoparticleSoil scienceMineralogyNanotechnologyMetallurgy

Abstract

fetched live from OpenAlex

The presence and transport of emerging Engineered Nano Particles (ENPs) in the environment is driven by combination of multiple factors comprising their size, charge and aggregation/agglomeration rate along with interactions with different soil types. Due to the complexity of the soil, it is difficult to associate an exact concentration with the possible transport pathways, interactions and transformation mechanisms. Major uncertainties arise with the increased number of extraction and filtration steps required for determining the exact toxicity doses of ENPs. Due to these issues, TiO2 and Ag behavior, characterization, transport, and environmental effects in soils are still not clear. In soils, TiO2 and Ag have been mainly reported to be present in the surroundings of point sources and are driven by their aggregation/agglomeration rate in combination with different soil types. TiO2 and Ag are mainly transported by interstitial water depending on their zeta-potential in the local soil. Along the transport route, TiO2 and Ag undergo alteration in dissolution, corrosion, redox reaction and coatings with the soil matrix. Their mobility is better across mineral soil in comparison to soil rich in organic colloids. The bioavailability gets modified and, in consequence, they are retained until complete degradation of the organic matrix. Depending on the soil matrix composition in terms of water content, minerals, and biological structure, the current most used methods for TiO2 and Ag characterization are FFFF and UV spectroscopy coupled with ICP-MS and LCMS/MS. The increased flux of TiO2 and Ag across soil is significant in understanding/accessing the viable threats, in particular their release affects the natural ecosystem.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.001
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.336
Threshold uncertainty score0.434

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0010.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.001
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.028
GPT teacher head0.261
Teacher spread0.233 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations127
Published2015
Admission routes2
Has abstractyes

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