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Record W2271066241 · doi:10.5194/acp-16-573-2016

Reactive nitrogen partitioning and its relationship to winter ozone events in Utah

2016· article· en· W2271066241 on OpenAlexaff
R. J. Wild, P. M. Edwards, T. S. Bates, R. C. Cohen, J. A. de Gouw, W. P. Dubé, J. B. Gilman, John W. Holloway, James P. Kercher, Abigail R. Koss, L. Lee, B. M. Lerner, R. McLaren, Patricia K. Quinn, J. M. Roberts, J. Stutz, Joel A. Thornton, Patrick R. Veres, C. Warneke, E. J. Williams, Cora J. Young, Bin Yuan, Kyle J. Zarzana, Steven S. Brown

Bibliographic record

VenueAtmospheric chemistry and physics · 2016
Typearticle
Languageen
FieldEarth and Planetary Sciences
TopicAtmospheric chemistry and aerosols
Canadian institutionsMemorial University of NewfoundlandYork University
FundersNational Oceanic and Atmospheric AdministrationU.S. Bureau of Land ManagementUtah Department of Environmental QualityUtah State University
KeywordsOzoneNOxReactive nitrogenTropospheric ozoneAtmospheric sciencesEnvironmental scienceNitrogen oxideNitrogenNitrogen dioxideNitrogen oxidesNitric acidAtmospheric chemistryAerosolTroposphereDaytimeChemistryEnvironmental chemistryMeteorologyGeographyGeologyInorganic chemistry

Abstract

fetched live from OpenAlex

High wintertime ozone levels have been observed in the Uintah Basin, Utah, a sparsely populated rural region with intensive oil and gas operations. The reactive nitrogen budget plays an important role in tropospheric ozone formation. Measurements were taken during three field campaigns in the winters of 2012, 2013 and 2014, which experienced varying climatic conditions. Average concentrations of ozone and total reactive nitrogen were observed to be 2.5 times higher in 2013 than 2012, with 2014 an intermediate year in most respects. However, photochemically active NO x (NO + NO 2 ) remained remarkably similar all three years. Nitric acid comprised roughly half of NO z ( ≡ NO y − NO x ) in 2013, with nighttime nitric acid formation through heterogeneous uptake of N 2 O 5 contributing approximately 6 times more than daytime formation. In 2012, N 2 O 5 and ClNO 2 were larger components of NO z relative to HNO 3 . The nighttime N 2 O 5 lifetime between the high-ozone year 2013 and the low-ozone year 2012 is lower by a factor of 2.6, and much of this is due to higher aerosol surface area in the high-ozone year of 2013. A box-model simulation supports the importance of nighttime chemistry on the reactive nitrogen budget, showing a large sensitivity of NO x and ozone concentrations to nighttime processes.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.001
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Observational · Consensus signal: Observational
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.130
Threshold uncertainty score0.259

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.001
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.001
Science and technology studies0.0010.000
Scholarly communication0.0000.000
Open science0.0000.001
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.013
GPT teacher head0.216
Teacher spread0.203 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designObservational
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations38
Published2016
Admission routes1
Has abstractyes

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