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Record W2272002727 · doi:10.1007/s13203-016-0146-1

Bitumen heavy oil upgrading by cavitation processing: effect on asphaltene separation, rheology, and metal content

2016· article· en· W2272002727 on OpenAlex

Why this work is in the frame

A frame that forgets how it found something cannot be audited. These are the routes that admitted this work.

affAt least one author lists a Canadian institution in the pinned OpenAlex snapshot.
fundA Canadian funder is recorded on the work.

Bibliographic record

VenueApplied Petrochemical Research · 2016
Typearticle
Languageen
FieldChemistry
TopicPetroleum Processing and Analysis
Canadian institutionsNational Research Council Canada
FundersNational Research Council Canada
KeywordsAsphalteneSonicationAsphaltCavitationRheologyMaterials scienceViscosityChemistryChemical engineeringComposite materialChromatographyOrganic chemistryThermodynamics

Abstract

fetched live from OpenAlex

Cavitation processing has been proposed as a greener alternative to solvent dilution or heat treatment of bitumen and other heavy oils to reduce viscosity and hence, improve transportability. The effect of acoustic cavitation under different conditions of sonication frequencies (low- to high- frequency range) and power inputs on asphaltene content, rheological changes, and metal content of bitumen was investigated in this study. Ultrasonic treatment resulted in a decrease in asphaltene content in bitumen that lead to lower viscosity and shear stress over a wide range of shear rates. Over the range of sonication frequencies investigated (20 kHz–1.1 MHz), the sonication frequency of 574 kHz with 50 % power input resulted in low asphaltene content and lower viscosity suitable for improved transportability. Further, comparison of different conditions of sonication frequencies and power inputs were carried out to investigate the effect of ultrasound on properties of asphaltene (elemental analysis and metal content). It was observed that the sonication treatment of bitumen under different conditions of frequencies and acoustic power decreased the H/C ratio. These results showed higher content of aromatic hydrogen and lower content of aliphatic hydrogen in bitumen treated under different conditions of sonication frequencies and intensity. Characterization of asphaltene performed using ICP-MS and TXRF, revealed lower metal content (Ni, Fe, and V) in the asphaltene phase of processed (sonicated) bitumen. The lowered metal content can be attributed to the reduced asphaltene formation as a result of sonication treatment of bitumen.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.001
metaresearch head score (Gemma)0.001
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.082
Threshold uncertainty score0.696

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0010.001
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.042
GPT teacher head0.350
Teacher spread0.308 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it