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Kinetic Modeling of the Biogenic Production of Coalbed Methane

2016· article· en· W2284964478 on OpenAlexafffund
Gouthami Senthamaraikkannan, Karen Budwill, Ian D. Gates, Sushanta K. Mitra, Vinay Prasad

Bibliographic record

VenueEnergy & Fuels · 2016
Typearticle
Languageen
FieldEngineering
TopicAnaerobic Digestion and Biogas Production
Canadian institutionsYork UniversityAlberta InnovatesUniversity of CalgaryUniversity of Alberta
FundersNatural Sciences and Engineering Research Council of CanadaCarbon Management Canada
KeywordsMethanogenesisAcetogenesisCoalbed methaneChemistryMethaneCoalAcidogenesisReaction rateAnaerobic digestionCoal miningOrganic chemistryCatalysis

Abstract

fetched live from OpenAlex

Biogenic production of coalbed methane under anaerobic conditions occurs through a large number of reactions involving a community of micro-organisms. We propose a kinetic scheme for this complicated reaction network using lumped species reacting in a series of enzymatic reaction blocks consisting of coal solubilization, hydrolysis, acidogenesis, acetogenesis, and methanogenesis. Among these pathways, acetoclastic methanogenesis is assumed to be dominant. Based on implications from experimental data, tryptone (a nitrogen rich nutrient used in the stimulation of methane production) is assumed to produce aromatic ring intermediates. Coal solubilization is described by a diffusion layer model. Monod kinetics are applied to model the enzymatic reaction rates, but the rate of methanogenesis is modeled with modified Monod kinetics to account for substrate inhibition. An analytical solution to the model is derived and its parametric sensitivity is investigated in different operating regions. Model parameters are estimated from data from various anaerobic bottle experiments conducted by us using nonlinear regression with the particle swarm optimization algorithm, and the model’s predictive ability has been validated for various coal samples from the literature, too. The predictive kinetic model thus established provides estimates of the concentration of products as well as intermediate species in the conversion of coal. The model can be used to optimize biogenic methane production from coal at different scales ranging from coreflooding experiments to the reservoir and field scales.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.027
Threshold uncertainty score0.164

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.011
GPT teacher head0.194
Teacher spread0.182 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations25
Published2016
Admission routes2
Has abstractyes

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