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Record W2289365991 · doi:10.1021/acs.jpcc.5b10711

Hydrogen Solubility of Magnetron Co-Sputtered FCC and BCC PdCuAu Thin Films

2016· article· en· W2289365991 on OpenAlex

Why this work is in the frame

A frame that forgets how it found something cannot be audited. These are the routes that admitted this work.

affAt least one author lists a Canadian institution in the pinned OpenAlex snapshot.
fundA Canadian funder is recorded on the work.

Bibliographic record

VenueThe Journal of Physical Chemistry C · 2016
Typearticle
Languageen
FieldMaterials Science
TopicCopper Interconnects and Reliability
Canadian institutionsInstitut National de la Recherche Scientifique
FundersNatural Sciences and Engineering Research Council of CanadaAir Liquide
KeywordsCavity magnetronMaterials scienceHydrogenSolubilityThin filmSputter depositionMetallurgyComposite materialNanotechnologyChemistrySputteringPhysical chemistryOrganic chemistry

Abstract

fetched live from OpenAlex

Palladium–copper–gold (PdCuAu) ternary alloy membranes are promising alternatives to pure palladium for the purpose of hydrogen separation processes. In the current work, PdCuAu ternary alloys were prepared by magnetron cosputtering deposition. All as-deposited samples showed face-centered cubic (fcc) structure in the composition range of study: 30 ≤ [Pd] ≤ 100, 0 ≤ [Cu] ≤ 66, and 0 ≤ [Au] ≤ 6 (in at%). The body-centered cubic (bcc) phase was prepared from the fcc samples by annealing for 4 h at 400 °C under Ar and was identified in alloys with Pd content between 40 and 46 at%. The hydrogen solubility was evaluated for both fcc and bcc phases using an electrochemical method and an electrochemical in situ X-ray diffraction method, respectively. The alloys’ hydrogen solubility increases with the lattice parameter and palladium content, and decreases with crystallite size and phase transition to bcc. In the same range of composition, the hydrogen solubility of the fcc and bcc phases vary in the same way with palladium content, suggesting that the latter factor is an important determinant of the hydrogen solubility in each phase.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.001
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.002
Threshold uncertainty score0.668

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0010.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.010
GPT teacher head0.247
Teacher spread0.238 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it