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Challenges in design of Kitaev materials: Magnetic interactions from competing energy scales

2016· article· en· 528 citations· W2293879704 on OpenAlex· 10.1103/physrevb.93.214431

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Canadian funderA Canadian agency funded it. The work may carry no Canadian affiliation at all.

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Opus teacher head0.044
GPT teacher head0.359
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Abstract

Much interest has emerged in the realization of materials with quantum spin liquid ground states, which would provide fertile ground for realizing exotic excitations. Three ``Kitaev'' spin liquid candidate materials have been proposed -- Na${}_{2}$IrO${}_{3}$, $\ensuremath{\alpha}$-RuCl${}_{3}$, and $\ensuremath{\alpha}$-Li${}_{2}$IrO${}_{3}$ -- and there has been many diverging proposals for the most relevant interactions. Here, the authors re-evaluate carefully the magnetic interactions in these materials, using nonperturbative exact diagonalization methods. The results clarify misconceptions in the literature and help estimate the potential for realizing the spin liquid state in real materials.

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The record

Venue
Physical review. B./Physical review. B
Topic
Advanced Condensed Matter Physics
Field
Physics and Astronomy
Canadian institutions
Funders
Natural Sciences and Engineering Research Council of CanadaChina Scholarship CouncilDeutsche Forschungsgemeinschaft
Keywords
AnisotropyPhysicsRange (aeronautics)Condensed matter physicsDiagonalCoupling (piping)Spin (aerodynamics)Statistical physicsQuantum spin liquidTheoretical physicsQuantum mechanicsMaterials scienceThermodynamicsMathematics
Has abstract in OpenAlex
yes