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Record W2301559491 · doi:10.1021/acs.jchemed.5b00059

Useful Material Efficiency Green Metrics Problem Set Exercises for Lecture and Laboratory

2015· article· en· W2301559491 on OpenAlexaff
John Andraos, Andrei Hent

Bibliographic record

VenueJournal of Chemical Education · 2015
Typearticle
Languageen
FieldEnvironmental Science
TopicChemistry and Chemical Engineering
Canadian institutionsUniversity of Toronto
Fundersnot available
KeywordsPlan (archaeology)Computer scienceMathematical proofSet (abstract data type)Tree (set theory)Simple (philosophy)ComputationTheoretical computer scienceAlgorithmMathematicsProgramming language

Abstract

fetched live from OpenAlex

A series of pedagogical problem set exercises are posed that illustrate the principles behind material efficiency green metrics and their application in developing a deeper understanding of reaction and synthesis plan analysis and strategies to optimize them. Rigorous, yet simple, mathematical proofs are given for some of the fundamental concepts, particularly how metrics for overall plan material performance are related to their composite counterparts for individual reactions. Throughout this exposition, whenever a synthesis scheme is examined, it is converted into a compact tree diagram that is used to depict plans of any degree of complexity (linear or convergent) as a means to conveniently keep track of all reagents, intermediates, reaction yields, stoichiometric coefficients, number of branches, number of reaction steps, and convergent steps. We demonstrate that such tree diagrams facilitate the computation of material efficiency metrics for any individual reaction in a plan as well as for the entire plan. We also show how such diagrams may be used to plan schedules for reaction operations when multiple linear branches are run concurrently. For brevity the Supporting Information contains full solutions to posed problems.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.003
metaresearch head score (Gemma)0.013
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Not applicable · Consensus signal: none
GenreCandidate signal: Methods · Consensus signal: Methods
Teacher disagreement score0.047
Threshold uncertainty score0.157

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0030.013
Meta-epidemiology (narrow)0.0030.001
Meta-epidemiology (broad)0.0010.001
Bibliometrics0.0010.001
Science and technology studies0.0010.001
Scholarly communication0.0020.003
Open science0.0020.004
Research integrity0.0020.005
Insufficient payload (model declined to judge)0.0470.009

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.009
GPT teacher head0.236
Teacher spread0.226 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designNot applicable
Domainnot available
GenreMethods

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations14
Published2015
Admission routes1
Has abstractyes

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