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Record W2305359896 · doi:10.1038/ncomms12519

Volume-wise destruction of the antiferromagnetic Mott insulating state through quantum tuning

2016· article· en· W2305359896 on OpenAlexafffund
Benjamin A. Frandsen, Lian Liu, Sky C. Cheung, Zurab Guguchia, R. Khasanov, E. Morenzoni, Timothy J. S. Munsie, Alannah M. Hallas, M. N. Wilson, Yipeng Cai, G. M. Luke, Bijuan Chen, Wenmin Li, Changqing Jin, Cui Ding, Shengli Guo, Fanlong Ning, T. Ito, Wataru Higemoto, Simon J. L. Billinge, Shoya Sakamoto, A. Fujimori, Taito Murakami, Hiroshi Kageyama, J. A. Alonso, Gabriel Kotliar, Masatoshi Imada, Y. J. Uemura

Bibliographic record

VenueNature Communications · 2016
Typearticle
Languageen
FieldMaterials Science
TopicMagnetic and transport properties of perovskites and related materials
Canadian institutionsCanadian Institute for Advanced ResearchMcMaster University
FundersOak Ridge National LaboratoryJapan Atomic Energy AgencyChinese Academy of SciencesBasic Energy SciencesNatural Sciences and Engineering Research Council of CanadaDivision of Materials ResearchMcMaster UniversityBrookhaven National LaboratoryU.S. Department of EnergySchweizerischer Nationalfonds zur Förderung der Wissenschaftlichen ForschungOffice of International Science and EngineeringOffice of ScienceCore Research for Evolutional Science and TechnologyMinistry of Education, Culture, Sports, Science and TechnologyNational Science Foundation
KeywordsCondensed matter physicsMott transitionMott insulatorAntiferromagnetismQuantum phase transitionMetal–insulator transitionStrongly correlated materialPhase transitionParamagnetismQuantumPhysicsMaterials scienceSuperconductivityHubbard modelQuantum mechanicsElectronElectrical resistivity and conductivity

Abstract

fetched live from OpenAlex

RENiO3 (RE=rare-earth element) and V2O3 are archetypal Mott insulator systems. When tuned by chemical substitution (RENiO3) or pressure (V2O3), they exhibit a quantum phase transition (QPT) between an antiferromagnetic Mott insulating state and a paramagnetic metallic state. Because novel physics often appears near a Mott QPT, the details of this transition, such as whether it is first or second order, are important. Here, we demonstrate through muon spin relaxation/rotation (μSR) experiments that the QPT in RENiO3 and V2O3 is first order: the magnetically ordered volume fraction decreases to zero at the QPT, resulting in a broad region of intrinsic phase separation, while the ordered magnetic moment retains its full value until it is suddenly destroyed at the QPT. These findings bring to light a surprising universality of the pressure-driven Mott transition, revealing the importance of phase separation and calling for further investigation into the nature of quantum fluctuations underlying the transition.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.001
Threshold uncertainty score0.003

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.018
GPT teacher head0.250
Teacher spread0.232 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations51
Published2016
Admission routes2
Has abstractyes

Explore more

Same venueNature CommunicationsSame topicMagnetic and transport properties of perovskites and related materialsFrench-language works237,207