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Record W2311050991 · doi:10.1021/acssuschemeng.5b01596

Microwave Synthesis and Melt Blending of Glycerol Based Toughening Agent with Poly(lactic acid)

2016· article· en· W2311050991 on OpenAlexafffund
Gildas Coativy, Manjusri Misra, Amar K. Mohanty

Bibliographic record

VenueACS Sustainable Chemistry & Engineering · 2016
Typearticle
Languageen
FieldMaterials Science
Topicbiodegradable polymer synthesis and properties
Canadian institutionsUniversity of Guelph
FundersOntario Ministry of Economic Development and InnovationNatural Sciences and Engineering Research Council of CanadaOntario Ministry of Agriculture, Food and Rural Affairs
KeywordsGlycerolMaterials scienceExtrusionPolylactic acidGlass transitionLactic acidSebacic acidChemical engineeringNuclear chemistryComposite materialPolymerOrganic chemistryPolymer chemistryChemistry

Abstract

fetched live from OpenAlex

High Resolution Image Download MS PowerPoint Slide Glycerol is a byproduct of the biodiesel industry. The target of the following work was to produce a biopolyester based on glycerol, and to blend it with poly(lactic acid) (PLA) to increase its ductility. Microwave synthesis was used to conduct the reactions of glycerol with a diacid (sebacic acid) and a monoacid (stearic acid) at 180 °C in bulk. Progress of the synthesis was stopped when a gel was obtained (after 3.45 h). The produced resin was found to be soluble in tetrahydrofuran (THF). The study of the product by infrared spectrometry showed an effective esterification of acids with glycerol. Calorimetric study evidenced a glass transition at −27 °C and a melting peak at 29 °C. PLA was then blended with various amounts of this biopolyester ranging from 0 to 20% via twin screw extrusion followed by injection molding. Morphologic characteristics of blends were studied by scanning electron microscopy. Biopolyester phases ranging from 100 nm to 10 μm were observed for all concentrations. In the particular case of 20% of biopolyester, micrometric phases greater than 10 μm in size were detected, leading to a decrease in mechanical performance. Tensile testing showed a ductile behavior for all concentrations higher than 5% of biopolyester, with an optimum performance achieved with 10% of biopolyester in which strain at break reached 93%.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.024
Threshold uncertainty score0.728

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.007
GPT teacher head0.175
Teacher spread0.168 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations50
Published2016
Admission routes2
Has abstractyes

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