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Record W2313300878 · doi:10.1021/ie3009023

Selective Recovery of Precious Metals from Acidic Leach Liquor of Circuit Boards of Spent Mobile Phones Using Chemically Modified Persimmon Tannin Gel

2012· article· en· W2313300878 on OpenAlex

Why this work is in the frame

A frame that forgets how it found something cannot be audited. These are the routes that admitted this work.

affAt least one author lists a Canadian institution in the pinned OpenAlex snapshot.

Bibliographic record

VenueIndustrial & Engineering Chemistry Research · 2012
Typearticle
Languageen
FieldEnvironmental Science
TopicRecycling and Waste Management Techniques
Canadian institutionsMemorial University of Newfoundland
FundersJapan Society for the Promotion of Science
KeywordsTanninPrecious metalPrinted circuit boardChemistryClosed circuitPulp and paper industryMaterials scienceWaste managementMetalComputer scienceOrganic chemistryFood scienceEngineering

Abstract

fetched live from OpenAlex

A tannin-based novel adsorbent, named “BTU-PT gel”, was prepared by immobilizing bisthiourea (BTU) ligand on persimmon tannin (PT) extract. The adsorption behaviors of precious metal ions along with other coexisting base metal ions onto BTU-PT gel were studied by batch and continuous column methods. The gel exhibited remarkable selectivity for precious metal ions such as Au(III), Pd(II), and Pt(IV) over base metal ions such as Cu(II), Fe(III), Ni(II), and Zn(II) in 1–5 mol dm –3 hydrochloric acid. The adsorption of precious metal ions on the present gel was found to obey the typical monolayer type of Langmuir model, and the maximum adsorption capacity of the adsorbent was evaluated as 5.18 mol kg –1 for Au(III), 1.80 mol kg –1 for Pd(II), and 0.67 mol kg –1 for Pt(IV). Combination of ion exchange, electrostatic interaction, and coordination through the thiocarbonyl group is the mechanism of adsorption of precious metals on BTU-PT gel. In the case of Au(III) adsorption, the adsorbed species was simultaneously reduced to elemental gold by abundant polyphenolic groups of the tannin matrix. Elution by using acidothiourea solution in continuous column experiment recovered the adsorbed precious metals almost quantitatively. The results of a potential reusability test of the gel for consecutive adsorption and elution cycles by continuous column experiment indicated that the gel was stable and regenerated with undiminished metal uptake capacity up to five cycles. The real time applicability of the adsorbent for the recovery of precious metals from real industrial liquor was evaluated from actual acidic leach liquor of printed circuit boards of spent mobile phones. The gel selectively adsorbed precious metal species but exhibited negligible affinity toward base metals present in the leach liquor. The BTU-PT gel is a potential adsorbent for selective recovery of precious metals from acidic leachate of spent mobile phones containing elevated concentrations of base metals.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.001
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.021
Threshold uncertainty score0.822

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0010.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.001
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.001
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.094
GPT teacher head0.320
Teacher spread0.227 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it