Periodic Macroporous Nanocrystalline Antimony-Doped Tin Oxide Electrode
Why this work is in the frame
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Bibliographic record
Abstract
Optically transparent and electrically conductive electrodes are ubiquitous in the myriad world of devices. They are an indispensable component of solar and photoelectrochemical cells, organic and polymer light emitting diodes, lasers, displays, electrochromic windows, photodetectors, and chemical sensors. The majority of the electrodes in such devices are made of large electronic band-gap doped metal oxides fashioned as a dense low-surface-area film deposited on a glass substrate. Typical transparent conducting oxide materials include indium-, fluorine-, or antimony-doped tin oxides. Herein we introduce for the first time a transparent conductive periodic macroporous electrode that has been self-assembled from 6 nm nanocrystalline antimony-doped tin oxide with high thermal stability, optimized electrical conductivity, and high quality photonic crystal properties, and present an electrochemically actuated optical light switch built from this electrode, whose operation is predicated on its unique combination of electrical, optical, and photonic properties. The ability of this macroporous electrode to host active functional materials like dyes, polymers, nanocrystals, and nanowires provides new opportunities to create devices with improved performance enabled by the large area, spatially accessible and electroactive internal surface.
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Full frame distilled prediction
Teacher imitationNot calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.
Codex and Gemma teacher scores by category
| Category | Codex | Gemma |
|---|---|---|
| Metaresearch | 0.000 | 0.000 |
| Meta-epidemiology (narrow) | 0.000 | 0.000 |
| Meta-epidemiology (broad) | 0.000 | 0.000 |
| Bibliometrics | 0.000 | 0.000 |
| Science and technology studies | 0.000 | 0.000 |
| Scholarly communication | 0.000 | 0.000 |
| Open science | 0.000 | 0.000 |
| Research integrity | 0.000 | 0.000 |
| Insufficient payload (model declined to judge) | 0.001 | 0.001 |
Machine scores (provisional)
The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.
Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.
score_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it