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Record W2316954273 · doi:10.1021/jp809905u

Dielectric Properties of Ga-Doped Na<sub>0.5</sub>K<sub>0.5</sub>NbO<sub>3</sub>

2009· article· en· W2316954273 on OpenAlexafffund
Eric Atamanik, Venkataraman Thangadurai

Bibliographic record

VenueThe Journal of Physical Chemistry C · 2009
Typearticle
Languageen
FieldMaterials Science
TopicFerroelectric and Piezoelectric Materials
Canadian institutionsUniversity of Calgary
FundersNatural Sciences and Engineering Research Council of Canada
KeywordsDielectricMaterials scienceDielectric spectroscopyAnalytical Chemistry (journal)Orthorhombic crystal systemMicrostructureCurie temperatureLattice constantGrain boundaryPerovskite (structure)Atmospheric temperature rangePowder diffractionDopingMineralogyDiffractionCondensed matter physicsCrystallographyCrystal structureChemistryComposite materialOpticsPhysical chemistryThermodynamicsOptoelectronics

Abstract

fetched live from OpenAlex

In this Article, we investigated the dielectric properties of B-site Ga-doped K 0.5 Na 0.5 NbO 3 (KNN) in air using AC impedance spectroscopy from room temperature to about 800 °C. Powder X-ray diffraction (PXRD) studies showed the formation of perovskite-type structure with orthorhombic symmetry, √2 a p × 4 a p × √2 a p (where a p is perovskite-type lattice constant) for x = 0.01, 0.1, and 0.13 members of Na 0.5 K 0.5 Nb 1− x Ga x O 3 . The PXRD result is similar to the parent KNN structure. AC impedance results showed mainly bulk contribution over the frequency range of 0.1 Hz to 1 MHz for the x = 0.01 member, while bulk and grain-boundary contributions were present for x > 0.01 in the same frequency range. Scanning electron microscopy was used to study the effect of microstructure change for Ga 3+ substitution in KNN. The inclusion of Ga 3+ in KNN showed a significant change in the microstructure. The dielectric properties of Na 0.5 K 0.5 Nb 1− x Ga x O 3 were enhanced by increasing the Ga 3+ content; among the compounds studied, the x = 0.1 member exhibited the highest dielectric constant and lowest dielectric loss at 1 MHz over the temperature range studied. All of the Na 0.5 K 0.5 Nb 1− x Ga x O 3 materials had a maximum dielectric constant at around 420 °C, which is consistent with other KNN ceramics reported in the literature and can be attributed to the Curie temperature. A small peak in the dielectric constant at around 220 °C was due to a structural phase transition.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.001
metaresearch head score (Gemma)0.001
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesMeta-epidemiology (narrow)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.010
Threshold uncertainty score1.000

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0010.001
Meta-epidemiology (narrow)0.0010.000
Meta-epidemiology (broad)0.0010.000
Bibliometrics0.0000.001
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0010.000
Research integrity0.0000.001
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.012
GPT teacher head0.216
Teacher spread0.204 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations29
Published2009
Admission routes2
Has abstractyes

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