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Record W2317835286 · doi:10.1021/jp2039674

Understanding Molecular Interactions of Asphaltenes in Organic Solvents Using a Surface Force Apparatus

2011· article· en· W2317835286 on OpenAlex

Why this work is in the frame

A frame that forgets how it found something cannot be audited. These are the routes that admitted this work.

affAt least one author lists a Canadian institution in the pinned OpenAlex snapshot.
fundA Canadian funder is recorded on the work.

Bibliographic record

VenueThe Journal of Physical Chemistry C · 2011
Typearticle
Languageen
FieldChemistry
TopicPetroleum Processing and Analysis
Canadian institutionsUniversity of Alberta
FundersNatural Sciences and Engineering Research Council of CanadaSyncrude
KeywordsAsphalteneSurface forces apparatusvan der Waals forceMicaHeptaneSteric effectsTolueneSurface forceChemistryLondon dispersion forceAdhesionIntermolecular forceAdsorptionChemical engineeringChemical physicsOrganic chemistryMaterials scienceMoleculeComposite material

Abstract

fetched live from OpenAlex

A surface force apparatus was used to study the intermolecular forces of asphaltenes in toluene and heptane. The repulsive interaction forces measured between two asphaltene surfaces in toluene were shown to have a steric nature and could be described by the Alexander–de Gennes theory on steric repulsion between two interacting polymer layers in good solvents at short separation distances under high compression forces. On the other hand, the adhesion forces measured between asphaltenes in heptane can be described by van der Waals forces, which are responsible for asphaltene aggregation and precipitation in paraffinic solvents. The asphaltene films adsorbed on mica were found to swell significantly in toluene but only moderately in heptane. In addition, an adhesion force was observed between an asphaltene surface and a mica surface in toluene. The results from this study provide an insight into the basic interaction mechanisms of asphaltenes in organic media and hence in crude oil and bitumen production.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.008
Threshold uncertainty score0.348

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.068
GPT teacher head0.287
Teacher spread0.219 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it