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Record W2318416965 · doi:10.1055/s-0032-1320750

Structure and biological activity of a cyclic lipodepsipeptide phaeofungin discovered with the Candida albicans fitness test

2012· article· en· W2318416965 on OpenAlexaff
John G. Ondeyka, Guy H. Harris, Kithsiri Herath, Deborah L. Zink, Fidel Ernesto Morales Vicente, Gerald F. Bills, Gonzalo Platas, A González de Val, Bin Jiang, Jennifer Nielsen Kahn, Stefan Galuska, R.A. Giacobbe, George K. Abruzzo, Emily Hickey, Paul Liberator, Deming Xu, Terry Roemer, Surinder Singh

Bibliographic record

VenuePlanta Medica · 2012
Typearticle
Languageen
FieldAgricultural and Biological Sciences
TopicEssential Oils and Antimicrobial Activity
Canadian institutionsMerck Canada Inc. (Canada)
Fundersnot available
KeywordsCandida albicansCorpus albicansDerivatizationCaspofunginAntifungalAntibiosisMicrobiologyStereochemistryFermentationBiologyBiochemistryChemistryBacteriaGeneticsChromatographyMass spectrometry

Abstract

fetched live from OpenAlex

Phaeofungin, a cyclic lipodepsipeptide, was isolated from a fermentation a Phaeosphaeria sp. (Phaeosphaeriaceae) from Spain. Antibiosis of the extract was recognized in an assay for C. albicans cell-wall perturbing agents. The extracts were chemogenomically assayed in the C. albicans fitness test (CaFT) that profiles the activities of antifungal agents. The CaFT profile overlapped with, but was differentiated from that of an antifungal lipodepsipeptide, phomafungin. Differences were confirmed when structure of phaeofungin was elucidated by spectroscopic methods including HRFTMS and 2D NMR. The amino acid identity and configuration were confirmed by acid hydrolysis followed by Marfey's derivatization. The antifungal activities of both lipodepsipeptides demonstrated phaeofungin synergizes with aureobasidin A and caspofungin leading to ATP leakage from cells of C. albicans.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Observational · Consensus signal: none
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.754
Threshold uncertainty score0.229

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.011
GPT teacher head0.202
Teacher spread0.190 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designObservational
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations0
Published2012
Admission routes1
Has abstractyes

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