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Record W2319300189 · doi:10.1021/ie303397y

Measurement of Heavy Oil and Bitumen Vapor Pressure for Fluid Characterization

2013· article· en· W2319300189 on OpenAlexafffundabout
Orlando Castellanos Diaz, F. F. Schoeggl, Harvey W. Yarranton, Marco A. Satyro

Bibliographic record

VenueIndustrial & Engineering Chemistry Research · 2013
Typearticle
Languageen
FieldEngineering
TopicPhase Equilibria and Thermodynamics
Canadian institutionsVirtual Materials Group (Canada)University of Calgary
FundersNatural Sciences and Engineering Research Council of CanadaVirtual Materials GroupUniversity of Calgary
KeywordsVapor pressureBoiling pointFraction (chemistry)AsphaltChemistryVacuum distillationDistillationExtrapolationAnalytical Chemistry (journal)AsphalteneMass fractionMaterials scienceChromatographyOrganic chemistryComposite material

Abstract

fetched live from OpenAlex

The prediction of heavy oil phase behavior, particularly with solvents, is sensitive to the characterization of the middle and heavy boiling point components of the oil. These components are typically characterized based on an extrapolation of distillation data. One method to test the extrapolated characterization is to model the vapor pressures of these fractions or residues containing these fractions. Unfortunately, the vapor pressures are too low to be reliably measured with conventional techniques. A new high vacuum static apparatus was designed and constructed for the measurement of vapor pressure of heavy oil and bitumen samples. The apparatus is capable of measuring pressures from 100 down to 0.1 Pa and temperatures in the range of 293.15–473.15 K. New procedures were developed to degas samples and obtain accurate vapor pressures at vacuum conditions. The apparatus was tested on n -hexadecane and naphthalene at temperatures between 303.15 and 363.15 K. The measured vapor pressures were, on average, all within 13% of the literature data. The vapor pressures of a Western Canadian bitumen sample (WC_BIT_B1) and three of its fractions were measured using the apparatus. The WC_BIT_B1 bitumen was modeled using the Advanced Peng–Robinson equation of state using a Gaussian extrapolation of its distillation curve for the maltene fraction and a Gamma molecular distribution for its asphaltene fraction. The measured vapor pressures were all predicted to within 3.5%.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.200
Threshold uncertainty score0.667

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.059
GPT teacher head0.272
Teacher spread0.213 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations11
Published2013
Admission routes3
Has abstractyes

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