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Record W2320069767 · doi:10.1021/jp212158a

Independent Control of Electron and Hole Localization in Core/Barrier/Shell Nanostructures

2012· article· en· W2320069767 on OpenAlexaff
Pooja Tyagi, Patanjali Kambhampati

Bibliographic record

VenueThe Journal of Physical Chemistry C · 2012
Typearticle
Languageen
FieldMaterials Science
TopicQuantum Dots Synthesis And Properties
Canadian institutionsMcGill University
Fundersnot available
KeywordsExcitonNanostructureElectronPhysicsBandwidth (computing)Shell (structure)Parameter spaceCondensed matter physicsMaterials scienceMolecular physicsOptoelectronicsNanotechnologyQuantum mechanicsTelecommunicationsComputer scienceMathematics

Abstract

fetched live from OpenAlex

By use of a two-band effective mass model and first-order perturbation theory, we demonstrate the capacity for complete spatial control over excitonic wave functions in core/barrier/shell nanostructures. By exploring parameter space with core size and barrier width as variables, we show that each exciton can be in a core-localized or shell-localized state (Type-I localization) and as well in a charge-separated state (Type-II localization). Furthermore, the width of each localization region in parameter space can be tuned by controlling material properties, providing design principles for nanostructures with desirable features for key applications. Depending on the localization regime of excitons, both radiative and nonradiative decay rates can be significantly enhanced or suppressed in these nanostructures, making them suitable for dual-color emission and for producing low threshold and broad bandwidth of optical gain.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.001
Threshold uncertainty score0.163

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.009
GPT teacher head0.231
Teacher spread0.222 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations24
Published2012
Admission routes1
Has abstractyes

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