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Record W2323531993 · doi:10.1149/1.3697583

Pit Propagation in Pure Aluminum Investigated via the 1D Artificial Pit Technique: Growth Regimes, Surface Morphology and Implications for Stability Criteria

2012· article· en· W2323531993 on OpenAlexaff
Anthony Cook, Dirk Engelberg, Nicholas Stevens, Nicholas Laycock, Stephen White, Majid Ghahari, Medhi Monir, N.J.H. Holroyd

Bibliographic record

VenueECS Transactions · 2012
Typearticle
Languageen
FieldMaterials Science
TopicAnodic Oxide Films and Nanostructures
Canadian institutionsUniversity of Toronto
Fundersnot available
KeywordsDissolutionOhmic contactMaterials scienceAluminiumSaturation (graph theory)KineticsMineralogyAnalytical Chemistry (journal)MetallurgyNanotechnologyChemistryPhysicsChromatographyMathematics

Abstract

fetched live from OpenAlex

The growth kinetics of various diameter 1D aluminum artificial pits were investigated under potential control in 1 mol dm-3 HCl. Pits of diameter ≥ 50 μm display mass transport control at high potentials, Ohmic growth at intermediate values with a transition to a further region of potential-independent dissolution at ca. 100 mV prior to repassivation. Optical and x-ray computed tomography observations of pit cross-sections suggest Ohmic propagation is associated with non-uniform dissolution over the pit surface. By contrast narrow diameter pits (25 μm) show no evidence of dissolution below their limiting current density and appear to grow without surface roughening until 10 - 20 mV before repassivation. Investigation of the nature of pit growth prior to this point via potential perturbation techniques confirmed that dissolution occurs under mass transport control. These observations support the hypothesis that sustained pit propagation requires a high degree of saturation, close to 100%, in AlCl3.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.001
Threshold uncertainty score0.002

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.027
GPT teacher head0.269
Teacher spread0.242 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations6
Published2012
Admission routes1
Has abstractyes

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Same venueECS TransactionsSame topicAnodic Oxide Films and NanostructuresFrench-language works237,207