MétaCan
Menu
Back to cohort
Record W2324010193 · doi:10.11159/jbb.2014.001

Zeolite Catalyzed Hydrolysis in Aqueous and Ionic Liquid Media

2014· article· en· W2324010193 on OpenAlexvenueno aff
Luisa M. Smallwood, Robert L. White

Bibliographic record

VenueJournal of Biomass to Biofuel · 2014
Typearticle
Languageen
FieldChemistry
TopicZeolite Catalysis and Synthesis
Canadian institutionsnot available
Fundersnot available
KeywordsCatalysisIonic liquidChemistryReactivity (psychology)HydrolysisAqueous solutionZeoliteCelluloseInorganic chemistrySolventIonic strengthIonic bondingOrganic chemistryIon

Abstract

fetched live from OpenAlex

Hydrolysis of ethyl acetate and starch in water and of cellulose in an ionic liquid by using HY and HZSM-5 solid acid catalysts are compared. In water, HZSM-5 is more active than HY. This trend is reversed in ionic liquid. Reactivity differences are explained based on interactions between solvent and catalyst acid site local environments, which depend on zeolite channel structure and Si/Al ratio. Greater hydrolysis reactivity is achieved when the ionic strength of the reaction media is high. This is a consequence of ion exchange, allowing for transfer of catalyst protons to the reaction media, where they can more effectively protonate ester and glycosidic functionalities. Water interacts more strongly with HY acid sites, presumably because the lower Si/Al ratio results in framework channels that are more hydrophilic.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.001
metaresearch head score (Gemma)0.001
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.041
Threshold uncertainty score0.659

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0010.001
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0010.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.008
GPT teacher head0.216
Teacher spread0.208 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations4
Published2014
Admission routes1
Has abstractyes

Explore more

Same venueJournal of Biomass to BiofuelSame topicZeolite Catalysis and SynthesisFrench-language works237,207