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Record W2327074322 · doi:10.1021/cm501826b

Chiral Periodic Mesoporous Organosilicas: Probing Chiral Induction in the Solid State

2014· article· en· W2327074322 on OpenAlexafffund
Michael W. A. MacLean, Thomas K. Wood, Gang Wu, Robert P. Lemieux, Cathleen M. Crudden

Bibliographic record

VenueChemistry of Materials · 2014
Typearticle
Languageen
FieldMaterials Science
TopicMesoporous Materials and Catalysis
Canadian institutionsQueen's University
FundersNatural Sciences and Engineering Research Council of CanadaQueen's UniversityGovernment of Ontario
KeywordsDopantChirality (physics)Mesoporous materialPolymerizationMaterials scienceSolid-stateMesoporous organosilicaMonomerDopingOrganic chemistryChemical engineeringChemistryMesoporous silicaPhysical chemistryPolymerCatalysisPhysicsChiral symmetryComposite material

Abstract

fetched live from OpenAlex

The production of a variety of PMO materials made with 1,1′-biphenylene monomers, and the inclusion of 1,1′-binaphthalene dopants is described. The effect of the point of attachment with regard to the biaryl axis was studied, and it was found that the highest level of chirality transfer is obtained when the biaryl axis is not restricted by the polymerization point. In addition, the actual loading of dopant was found to vary considerably depending on the synthesis procedure, and the effect of dopant, even at low level, was magnified under basic conditions when more ordered materials are produced.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.002
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesInsufficient payload (model declined to judge)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.002
Threshold uncertainty score0.999

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0020.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0010.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0010.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0020.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.010
GPT teacher head0.230
Teacher spread0.221 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations23
Published2014
Admission routes2
Has abstractyes

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