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Record W2327218840 · doi:10.1021/sc500353v

Toughened Sustainable Green Composites from Poly(3-hydroxybutyrate-<i>co</i>-3-hydroxyvalerate) Based Ternary Blends and Miscanthus Biofiber

2014· article· en· W2327218840 on OpenAlexafffund
Kunyu Zhang, Manjusri Misra, Amar K. Mohanty

Bibliographic record

VenueACS Sustainable Chemistry & Engineering · 2014
Typearticle
Languageen
FieldMaterials Science
Topicbiodegradable polymer synthesis and properties
Canadian institutionsUniversity of Guelph
FundersOntario Ministry of Economic Development and InnovationNatural Sciences and Engineering Research Council of CanadaOntario Ministry of Agriculture, Food and Rural Affairs
KeywordsMaterials scienceComposite materialToughnessTernary operationReactive extrusionIzod impact strength testNatural rubberDynamic mechanical analysisSISALScanning electron microscopeExtrusionUltimate tensile strengthPolymer

Abstract

fetched live from OpenAlex

High Resolution Image Download MS PowerPoint Slide Novel green composites with an excellent balance of properties were successfully fabricated from poly(3-hydroxybutyrate- co -3-hydroxyvalerate) (PHBV) based renewable ternary blends and miscanthus through a cost-efficient reactive extrusion process. The ternary blend of PHBV with poly(butylene adipate- co -terephthalate) (PBAT) and epoxidized natural rubber (ENR) was engineered as a high toughening matrix for the natural fiber composites using dicumyl peroxide (DCP) as the reactive compatibilizer. The addition of miscanthus fibers into the matrix significantly enhanced its stiffness and thermal resistance while still keeping a good toughness. A high value of impact strength up to 240.5 J/m was still achieved even with 20 wt % miscathus added. The mechanical modulus of the composites were also analyzed using mathematical models including rule of mixtures (ROM), inverse rule of mixtures (IROM), and the Tsai–Pagano equations. In the multiphase blends and composites, ENR played unique dual roles as an effective coupling agent and impact modifier in the presence of DCP. Scanning electron microscopy (SEM) results indicated good interfacial adhesion among the different phases in the composites, which played a vital role in improving the strength and toughness of the materials. At the same time, balanced melt viscosity and density were also achieved for the composites, which are important for wide application.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesMeta-epidemiology (narrow)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.039
Threshold uncertainty score1.000

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0010.001
Meta-epidemiology (broad)0.0010.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0010.001
Open science0.0010.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.005
GPT teacher head0.181
Teacher spread0.176 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations77
Published2014
Admission routes2
Has abstractyes

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