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Thermodynamic Modeling of Chiral Compounds Solubility Using Correlative and Predictive Models

2015· article· en· W2329945655 on OpenAlexvenueno aff
Morteza Salimi, Bahman ZareNezhad, Hossein Fakhraian, Ebrahim Choobdari

Bibliographic record

VenueJournal of Applied Solution Chemistry and Modeling · 2015
Typearticle
Languageen
FieldEngineering
TopicPhase Equilibria and Thermodynamics
Canadian institutionsnot available
Fundersnot available
KeywordsUNIQUACNon-random two-liquid modelUNIFACSolubilityChemistryThermodynamicsActivity coefficientIntermolecular forceSolventOrganic chemistryAqueous solution

Abstract

fetched live from OpenAlex

Many intermolecular forces and parameters affect the solubility of a compound in a solvent. Various thermodynamic models are presented to predict these parameters and determine solid liquid equilibrium data. By selecting suitable thermodynamic model for solubility modeling, calculation error is reduced and the results will be closer to the experimental data. Herein, the ability of two predictive and two correlative models in solubility modeling of chiral compounds is investigated. Thus, solubility of pure and racemic forms of chiral Ketamine, Mandelic acid and 3-Chloromandelic acid is evaluated using UNIQUAC and NRTL models. The solubility modeling of pure and racemic forms of Ketamine in Ethanol is also determined by UNIFAC and NRTL-SAC models. There are good agreement between experimental data and results of NRTL and UNIQUAC models. Predictive NRTL-SAC model shows smaller deviation than UNIFAC in solubility determination of pure and racemic form of Ketamine.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Simulation or modeling · Consensus signal: Simulation or modeling
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.464
Threshold uncertainty score0.700

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.039
GPT teacher head0.243
Teacher spread0.204 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designSimulation or modeling
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations1
Published2015
Admission routes1
Has abstractyes

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