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Record W2331023358 · doi:10.1021/jp508629d

Reflection and Absorption Spectra of Silver Nanocubes on a Dielectric Substrate: Anisotropy, Angle, and Polarization Dependencies

2014· article· en· W2331023358 on OpenAlexafffund
Adam Bottomley, Anatoli Ianoul

Bibliographic record

VenueThe Journal of Physical Chemistry C · 2014
Typearticle
Languageen
FieldMaterials Science
TopicGold and Silver Nanoparticles Synthesis and Applications
Canadian institutionsCarleton University
FundersNatural Sciences and Engineering Research Council of Canada
KeywordsMaterials scienceMolecular physicsAnisotropyDielectricSpectral lineAbsorption (acoustics)OpticsWavelengthSurface plasmon resonanceDipoleResonance (particle physics)OptoelectronicsChemistryNanoparticleAtomic physicsNanotechnology

Abstract

fetched live from OpenAlex

Angle and polarization dependent UV–visible reflection and transmission spectra were measured for monolayers of weakly interacting silver nanocubes (of 40 and 80 nm edge lengths) supported by thin films of titanium oxide on glass utilizing both front and rear geometries with respect to the incident radiation. The supporting substrate mediates the hybridization of dipolar and quadrupolar plasmon resonances. From the spectra absolute extinction and absorption cross sections for supported silver nanocubes were determined. A strong angle dependence of the extinction and reflection spectra for p- but not s-polarized light was observed. This dependence is considerably more pronounced for the hybridized quadrupolar resonance of the 40 nm cubes. When illuminated from the rear, a significantly stronger absorption of light by the dipolar but not the quadrupolar resonance occurs for both cube sizes. Such absorption anisotropy could result from the wavelength dependent constructive or destructive interference between incident and scattered light from the nanocubes. This study demonstrates the impact of a dielectric substrate on the optical properties of novel plasmonic materials.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.002
Threshold uncertainty score0.006

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.001
Insufficient payload (model declined to judge)0.0020.001

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.010
GPT teacher head0.228
Teacher spread0.218 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations24
Published2014
Admission routes2
Has abstractyes

Explore more

Same venueThe Journal of Physical Chemistry CSame topicGold and Silver Nanoparticles Synthesis and ApplicationsFrench-language works237,207