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Record W2331100735 · doi:10.1021/ie501032j

Modeling and Simulation of a Multibed Industrial Hydrotreater with Vapor–Liquid Equilibrium

2014· article· en· W2331100735 on OpenAlexaff
Anton Alvarez‐Majmutov, Jinwen Chen

Bibliographic record

VenueIndustrial & Engineering Chemistry Research · 2014
Typearticle
Languageen
FieldEngineering
TopicCatalysis and Hydrodesulfurization Studies
Canadian institutionsNatural Resources Canada
Fundersnot available
KeywordsHydrodesulfurizationThermodynamicsVaporizationPlug flowChemistryNuclear engineeringMaterials scienceCatalysisOrganic chemistry

Abstract

fetched live from OpenAlex

Dealing with vapor–liquid equilibrium (VLE) in hydrotreating reactors is a major obstacle to realistic process simulation. The present study focused on the modeling and simulation of a commercial light-cycle-oil (LCO) hydrotreater with rigorous vapor–liquid equilibrium (VLE) calculations. The hydrotreater was represented as a one-dimensional plug-flow adiabatic reactor with interbed gas quenching. The model accounted for the hydrodesulfurization (HDS) and hydrodearomatization (HDA) reactions. VLE calculations were performed in situ with a calibrated flash calculation program developed in-house specifically for hydrogen–petroleum systems. Significant differences in reactor temperature profiles, hydrotreating conversions, fluid rates, and phase compositions were observed between the simulations with and without VLE. Analysis of the effect of temperature indicated that reactor performance depends heavily on the axial temperature distribution, which is established based on the catalyst bed layout and the selection of bed inlet temperatures. It was observed that, although conversion levels were improved at higher inlet temperatures, there was an increase in quenching gas requirement, vaporization rate, and the formation of high-temperature zones toward the inlet of the reactor. In a similar manner, pressure was found to increase hydrotreating performance markedly but with an extensive heat release. Verification of plug-flow and full-catalyst-wetting conditions during the simulations confirmed that all criteria were satisfied in this study.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.001
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Simulation or modeling · Consensus signal: Simulation or modeling
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.028
Threshold uncertainty score0.804

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0010.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.001
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.078
GPT teacher head0.296
Teacher spread0.219 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designSimulation or modeling
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations19
Published2014
Admission routes1
Has abstractyes

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