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Record W2331475905 · doi:10.1021/jp2108957

Subtle Photochemical Behavior in Ferroin–Bromate–Benzoquinone Reaction

2011· article· en· W2331475905 on OpenAlexaff
Jun Li, Jichang Wang

Bibliographic record

VenueThe Journal of Physical Chemistry A · 2011
Typearticle
Languageen
FieldChemistry
TopicPhotochemistry and Electron Transfer Studies
Canadian institutionsUniversity of Windsor
Fundersnot available
KeywordsBromatePhotochemistryChemistryOrganic chemistryIon

Abstract

fetched live from OpenAlex

This study investigated the photochemical behavior of the ferroin-bromate-benzoquinone reaction in a batch system, in which the reduction of ferriin was dominated by bromide ions rather than by organic substrates as known in most of bromate oscillators. The chemical oscillations exhibited ultrasensitive response to illumination, where both the oscillation frequency and lifetime were significantly increased by ceiling light with an intensity of less than 20 μW/cm(2). As the light intensity was increased, the influence of light evolved from constructive to inhibitory. At a constant illumination, the influence of light also underwent a transition from constructive to inhibitory when the acid concentration was increased from 0.03 to 0.09 M. NMR measurements and absorption spectroscopy indicated photoenhanced bromination of benzoquinone and photoenhanced reduction of ferriin by bromide ions.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.017
Threshold uncertainty score0.741

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0010.000
Research integrity0.0000.001
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.022
GPT teacher head0.250
Teacher spread0.227 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations4
Published2011
Admission routes1
Has abstractyes

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