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Record W2333311425 · doi:10.2166/wqrjc.2014.031

Computational modeling of UV photocatalytic reactors: model development, evaluation, and application

2014· article· en· W2333311425 on OpenAlexaff
J. Herrera, Madjid Mohseni, Fariborz Taghipour

Bibliographic record

VenueWater Quality Research Journal · 2014
Typearticle
Languageen
FieldEnergy
TopicTiO2 Photocatalysis and Solar Cells
Canadian institutionsUniversity of British Columbia
Fundersnot available
KeywordsIrradianceComputational fluid dynamicsLaminar flowReynolds stressPhotocatalysisTurbulenceMass transferMaterials scienceMechanicsNuclear engineeringChemistryEnvironmental sciencePhysicsEngineeringOpticsOrganic chemistryCatalysis

Abstract

fetched live from OpenAlex

A computational model for simulating the performance of immobilized photocatalytic ultraviolet (UV) reactors used for water treatment was developed, experimentally evaluated, and applied to reactor design optimization. This model integrated hydrodynamics, species mass transport, chemical reaction kinetics, and irradiance distribution within the reactor. Among different hydrodynamic models evaluated against experimental data, the laminar, Abe–Kondoh–Nagano, and Reynolds stress turbulence models showed better performance (errors <5%, 12%, and 20%, respectively) in terms of external mass transfer and surface reaction prediction capabilities at different hydrodynamic conditions. A developed finite-volume-based UV lamp emission model was able to predict, with errors of less than 5%, near- and far-field irradiance measurements. Combining all these models, the integrated computational fluid dynamics (CFD)-based model was able to successfully predict the photocatalytic degradation rate of model pollutants (benzoic acid and 2,4-D) in various configurations of annular reactors and UV lamp sizes, over a wide range of hydrodynamic conditions (350 < Re < 11,000). In addition, the integrated model was used in combination with a Taguchi design of experiments method to perform reactor design optimization. Following this approach, a base case annular reactor design was modified to obtain a 50% more efficient design.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.001
metaresearch head score (Gemma)0.001
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Simulation or modeling · Consensus signal: Simulation or modeling
GenreCandidate signal: Empirical · Consensus signal: none
Teacher disagreement score0.011
Threshold uncertainty score0.021

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0010.001
Meta-epidemiology (narrow)0.0010.000
Meta-epidemiology (broad)0.0010.001
Bibliometrics0.0000.001
Science and technology studies0.0010.000
Scholarly communication0.0010.001
Open science0.0020.001
Research integrity0.0010.001
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.151
GPT teacher head0.410
Teacher spread0.258 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designSimulation or modeling
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations16
Published2014
Admission routes1
Has abstractyes

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