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Record W2340665656 · doi:10.1021/acssuschemeng.6b00481

What Are the Major Components in Steam Pretreated Lignocellulosic Biomass That Inhibit the Efficacy of Cellulase Enzyme Mixtures?

2016· article· en· W2340665656 on OpenAlexafffund
Rui Zhai, Jinguang Hu, Jack Saddler

Bibliographic record

VenueACS Sustainable Chemistry & Engineering · 2016
Typearticle
Languageen
FieldEngineering
TopicBiofuel production and bioconversion
Canadian institutionsUniversity of British Columbia
FundersNatural Sciences and Engineering Research Council of CanadaChina Scholarship Council
KeywordsCellulaseLignocellulosic biomassBiomass (ecology)ChemistryPulp and paper industryBiofuelEnzymeLigninCelluloseBiotechnologyFood scienceOrganic chemistryAgronomyBiology

Abstract

fetched live from OpenAlex

Any pretreat process used on lignocellulosic substrates, such as steam pretreatment, although opening up and enhancing access to the cellulose, will typically generate inhibitory compounds (i.e., soluble mono/oligomeric sugars, phenolics, furans, extractives, etc.) that limit or restrict the efficiency of enzyme mediated cellulose hydrolysis. In the work reported here, the major groups of inhibitors derived from various, “real-life” steam pretreated lignocellulosic biomass were identified and their inhibitory effects on the rate and extent of enzymatic hydrolysis were assessed. It was apparent that monomeric sugars and phenolics inhibited the hydrolytic potential of the cellulases most severely, with sugar accounting for the majority of the decrease. The inhibitory effect of the monomeric sugars was consistent and concentration (but not composition) dependent throughout the time course of hydrolysis. In contrast, the influence of the phenolics was substrate dependent and more harmful at the later stage of hydrolysis. Surprisingly, the oligomeric sugars derived after steam pretreatment of woody biomass showed little influence on the hydrolytic potential of cellulase enzymes.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.007
Threshold uncertainty score0.696

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.009
GPT teacher head0.181
Teacher spread0.172 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations91
Published2016
Admission routes2
Has abstractyes

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