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Record W2343505850 · doi:10.1186/s40929-016-0005-4

Electric ion dispersion as a new type of mass spectrometer

2016· article· en· W2343505850 on OpenAlexaff
M. J. Lindstrom, Iain R. Moyles, Kevin Ryczko

Bibliographic record

VenueMathematics-in-Industry Case Studies · 2016
Typearticle
Languageen
FieldChemistry
TopicMass Spectrometry Techniques and Applications
Canadian institutionsUniversity of Ontario Institute of Technology
Fundersnot available
KeywordsMass spectrometryQuadrupoleQuadrupole mass analyzerElectromagnetic massPhysicsElectric fieldComputational physicsSecondary ion mass spectrometryMagnetic fieldDispersion (optics)SpectrometerAnalytical Chemistry (journal)ChemistryAtomic physicsOpticsClassical mechanicsChromatography

Abstract

fetched live from OpenAlex

At the 2014 Fields-MPrime Industrial Problem Solving Workshop, PerkinElmer presented a design problem for mass spectrometry. Traditionally, mass spectrometry is done via three methods: using magnetic fields to deflect charged particles whereby different masses bend differently; using a time-of-flight procedure where particles of different mass arrive at different times at a target; and using an electric quadrupole that filters out all masses except for one very narrow band. The challenge posed in the problem was to come up with a new design for mass spectrometry that did not involve magnetic fields and where mass fractions could be measured in an entire sample on a continuous basis. We found that by sending the sample particles down a channel of line charges oscillations would be induced with a spatial wavelength being mass dependent thereby allowing different masses to be separated spatially and potentially detected on a continuous basis, without the use of magnetic fields. In this paper, we present the analysis of our design and illustrate how this principle could be used for mass spectrometry.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.003
metaresearch head score (Gemma)0.004
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: none
Teacher disagreement score0.004
Threshold uncertainty score0.015

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0030.004
Meta-epidemiology (narrow)0.0010.001
Meta-epidemiology (broad)0.0010.000
Bibliometrics0.0010.001
Science and technology studies0.0010.002
Scholarly communication0.0020.003
Open science0.0020.002
Research integrity0.0020.001
Insufficient payload (model declined to judge)0.0040.001

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.040
GPT teacher head0.324
Teacher spread0.284 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations0
Published2016
Admission routes1
Has abstractyes

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