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Record W2344532002 · doi:10.1021/acs.iecr.6b00376

Polymer Coating over Solid Particles with <i>In Situ</i> Thermal Curing

2016· article· en· W2344532002 on OpenAlexafffund
Shimiao Zhang, L. So, Santiago Faucher, Li Xi

Bibliographic record

VenueIndustrial & Engineering Chemistry Research · 2016
Typearticle
Languageen
FieldChemistry
TopicPetroleum Processing and Analysis
Canadian institutionsHatch (Canada)McMaster University
FundersNatural Sciences and Engineering Research Council of Canada
KeywordsCoatingHexamethylenetetramineMaterials scienceCuring (chemistry)PolymerComposite materialChemical engineeringRheologyMelting point

Abstract

fetched live from OpenAlex

Solid particles coated by cross-linked polymer layers find applications in many areas, including hydraulic fracturing operations. In this study, a hot-melt resin coating process for solid particles is developed and optimized for hydraulic fracturing applications. Phenolic resin is used to coat the particles above its melting point and is subsequently cured in situ by hexamethylenetetramine (HMTA). The coating quality is then characterized by the surface morphology, acid solubility, and crush resistance of the resin-coated particles. The effects of various operating parameters on the coating performance are systematically studied. Among them, temperature is shown to play an especially important role. The coating process involves intricate coupling between resin rheology, HMTA mass transfer, and curing kinetics, all of which are profoundly influenced by temperature. Different constant temperature levels as well as controlled temperature ramps are investigated, and the results show a complex dependence. Higher temperature leads to stronger coating layers with better barrier properties, whereas lower temperature is preferable for better surface morphology. These two trends can be partially reconciled with ramping temperature profiles; the improvement is, however, eventually limited by the rate of heat transfer. This study not only provides insight into the physical and chemical processes underlying the resin coating operation, it also demonstrates a generalizable strategy suitable for various particle coating processes.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.001
Threshold uncertainty score0.003

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.046
GPT teacher head0.307
Teacher spread0.261 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations12
Published2016
Admission routes2
Has abstractyes

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