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Thermal Crackability/Processability of Oils and Residua

2016· article· en· W2345661947 on OpenAlexafffund
Lante Carbognani Ortega, Josune Carbognani, Estrella Rogel, César Ovalles, Janie Vien, Harris Morazan, Francisco López-Linares, Pedro Pereira‐Almao

Bibliographic record

VenueEnergy & Fuels · 2016
Typearticle
Languageen
FieldChemistry
TopicPetroleum Processing and Analysis
Canadian institutionsUniversity of Calgary
FundersNatural Sciences and Engineering Research Council of CanadaHunan Provincial Science and Technology DepartmentCanada Foundation for InnovationChevron
KeywordsThermalMaterials scienceChemistryEnvironmental scienceChemical engineeringEngineeringThermodynamicsPhysics

Abstract

fetched live from OpenAlex

The maximum potential for producing light ends under a set of operational parameters for oil feedstocks is termed “crackability”. When constrained by the appearance of undesirable solid phases, the term “processability” applies to the potential of light ends production. These parameters were correlated with the thermal maturity of the samples. Thermal maturity was inferred from two proposed indicators: the first one was based on the “delta solubility parameter” (ΔPS) and the second was based on differential heavy hydrocarbon abundances determined by high-temperature simulated distillation (Δ%(C44–C100)). A set of 36 samples that was comprised of oils, distillation residua, and thermally cracked residua was studied. Samples with increased thermal maturity were found to decrease their crackability/processability. Samples with high solubility parameter (ΔPS), low Δ%(C44–C100), and low molecular weight were found to have increased thermal maturity. Attempts to correlate saturates, aromatics, resins, and asphaltenes (SARA) group-type distributions with thermal maturity were not successful. Highly paraffinic samples were found to deviate from the determined behavior of studied samples. Application of the proposed crackability/processability indicators to thermal processing under batch, semi-batch, and continuous setup conditions, was found to describe most of the experimentally determined results.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.001
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.001
Threshold uncertainty score0.003

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.001
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0010.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.008
GPT teacher head0.225
Teacher spread0.216 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations5
Published2016
Admission routes2
Has abstractyes

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