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Record W2443847915 · doi:10.1021/acs.jpcc.6b03850

Probing the Adsorption of Polycyclic Aromatic Compounds onto Water Droplets Using Molecular Dynamics Simulations

2016· article· en· W2443847915 on OpenAlex

Why this work is in the frame

A frame that forgets how it found something cannot be audited. These are the routes that admitted this work.

affAt least one author lists a Canadian institution in the pinned OpenAlex snapshot.
fundA Canadian funder is recorded on the work.

Bibliographic record

VenueThe Journal of Physical Chemistry C · 2016
Typearticle
Languageen
FieldChemistry
TopicAdvanced Physical and Chemical Molecular Interactions
Canadian institutionsUniversity of Alberta
FundersCanadian Centre for Clean Coal/Carbon and Mineral Processing TechnologiesNatural Sciences and Engineering Research Council of Canada
KeywordsAdsorptionHeptaneMolecular dynamicsChemical physicsTolueneChemistryMoleculeRADIUSHydrodynamic radiusCurvatureChemical engineeringPhysical chemistryComputational chemistryOrganic chemistryAqueous solutionMicelle

Abstract

fetched live from OpenAlex

A series of molecular dynamics (MD) simulations were performed to probe the adsorption behaviors of polycyclic aromatic compounds (PACs) from n -heptane and toluene onto water droplets. In n -heptane, the simulations revealed distinct adsorbed structures of PAC molecules on the water droplets with different sizes. In the system with a small water droplet (radius 1.86 nm), the adsorbed PAC aggregate renders a straight one-dimensional (1D) structure; contrarily, in the presence of a large water droplet (radius 3.10 nm), a bent 1D structure of nonzero curvature is formed. Such size effect is a result from the delicate balance between the deformation energy required for adsorption and the available attractions between the PAC and water molecules. While the adsorbed structures are sensitive to the size of the water droplet at relatively low PAC concentration in n -heptane, the size effect in toluene is only prominent when the concentration of PAC molecules is sufficiently high.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.019
Threshold uncertainty score0.290

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.010
GPT teacher head0.255
Teacher spread0.246 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it