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Record W2463282523 · doi:10.1002/adfm.201602155

Long‐Range Domain Structure and Symmetry Engineering by Interfacial Oxygen Octahedral Coupling at Heterostructure Interface

2016· article· en· W2463282523 on OpenAlexafffund
Zhaoliang Liao, Robert J. Green, Nicolas Gauquelin, S. Macke, Lin Li, J. Gonnissen, Ronny Sutarto, Evert Pieter Houwman, Zhicheng Zhong, Sandra Van Aert, Johan Verbeeck, G. A. Sawatzky, Mark Huijben, Gertjan Koster, Guus Rijnders

Bibliographic record

VenueAdvanced Functional Materials · 2016
Typearticle
Languageen
FieldEngineering
TopicPerovskite Materials and Applications
Canadian institutionsCanadian Light Source (Canada)University of British Columbia
FundersWestern Economic Diversification CanadaCanadian Institutes of Health ResearchNatural Sciences and Engineering Research Council of CanadaEuropean CommissionVlaamse regeringNederlandse Organisatie voor Wetenschappelijk OnderzoekFonds Wetenschappelijk OnderzoekCanadian Light Source
KeywordsMaterials scienceHeterojunctionPerovskite (structure)EpitaxyOctahedronCondensed matter physicsSymmetry (geometry)Coupling (piping)Chemical physicsSubstrate (aquarium)Thin filmCrystal structureCrystallographic point groupStrain engineeringCrystallographyNanotechnologyOptoelectronicsComposite materialLayer (electronics)ChemistrySiliconGeometryPhysics

Abstract

fetched live from OpenAlex

In epitaxial thin film systems, the crystal structure and its symmetry deviate from the bulk counterpart due to various mechanisms such as epitaxial strain and interfacial structural coupling, which is accompanyed by a change in their properties. In perovskite materials, the crystal symmetry can be described by rotations of sixfold coordinated transition metal oxygen octahedra, which are found to be altered at interfaces. Here, it is unraveled how the local oxygen octahedral coupling at perovskite heterostructural interfaces strongly influences the domain structure and symmetry of the epitaxial films resulting in design rules to induce various structures in thin films using carefully selected combinations of substrate/buffer/film. Very interestingly it is discovered that these combinations lead to structure changes throughout the full thickness of the film. The results provide a deep insight into understanding the origin of induced structures in a perovskite heterostructure and an intelligent route to achieve unique functional properties.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesInsufficient payload (model declined to judge)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.017
Threshold uncertainty score1.000

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.004
GPT teacher head0.190
Teacher spread0.186 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations32
Published2016
Admission routes2
Has abstractyes

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